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@ARTICLE{Kalikka:819868,
author = {Kalikka, J. and Akola, Jaakko and Jones, Robert O.},
title = {{C}rystallization processes in the phase change material
{G}e$_{2}${S}b$_{2}${T}e$_{5}$: {U}nbiased density
functional/molecular dynamics simulations},
journal = {Physical review / B},
volume = {94},
number = {13},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2016-05447},
pages = {134105},
year = {2016},
abstract = {Three extensive density functional/molecular dynamics
simulations of the crystallization of amorphous Ge2Sb2Te5
(460 atoms) [Phys. Rev. B 90, 184109 (2014)] have been
completed with simulation times of up to 8.2 ns. Together
with the results of earlier simulations with and without a
crystallite seed, the results clarify essential features of
a complicated process. They emphasize, in particular, the
stochastic nature of crystallization, the effect of bond
orientations and percolation, and the importance of extended
simulations of sufficiently large samples. This is
particularly evident in describing the role of crystallites
that can merge to form larger units or hinder complete
crystallization by the formation of grain boundaries. The
total pair distribution functions for the final structures
are compared with available neutron and x-ray diffraction
data},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000386089600001},
doi = {10.1103/PhysRevB.94.134105},
url = {https://juser.fz-juelich.de/record/819868},
}