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000819969 1001_ $$0P:(DE-HGF)0$$aFrandsen, Benjamin A.$$b0$$eCorresponding author
000819969 245__ $$aLocal atomic and magnetic structure of dilute magnetic semiconductor (Ba , K) (Zn , Mn)$_{2}$ As$_{2}$
000819969 260__ $$aWoodbury, NY$$bInst.$$c2016
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000819969 520__ $$aWe have studied the atomic and magnetic structure of the dilute ferromagnetic semiconductor system (Ba,K)(Zn,Mn)2As2 through atomic and magnetic pair distribution function analysis of temperature-dependent x-ray and neutron total scattering data. We detected a change in curvature of the temperature-dependent unit cell volume of the average tetragonal crystallographic structure at a temperature coinciding with the onset of ferromagnetic order. We also observed the existence of a well-defined local orthorhombic structure on a short length scale of ≲5Å, resulting in a rather asymmetrical local environment of the Mn and As ions. Finally, the magnetic PDF revealed ferromagnetic alignment of Mn spins along the crystallographic c axis, with robust nearest-neighbor ferromagnetic correlations that exist even above the ferromagnetic ordering temperature. We discuss these results in the context of other experiments and theoretical studies on this system.
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000819969 7001_ $$0P:(DE-HGF)0$$aBillinge, Simon J. L.$$b8
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