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| 001 | 819969 | ||
| 005 | 20240619092110.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.94.094102 |2 doi |
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| 100 | 1 | _ | |a Frandsen, Benjamin A. |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Local atomic and magnetic structure of dilute magnetic semiconductor (Ba , K) (Zn , Mn)$_{2}$ As$_{2}$ |
| 260 | _ | _ | |a Woodbury, NY |c 2016 |b Inst. |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a We have studied the atomic and magnetic structure of the dilute ferromagnetic semiconductor system (Ba,K)(Zn,Mn)2As2 through atomic and magnetic pair distribution function analysis of temperature-dependent x-ray and neutron total scattering data. We detected a change in curvature of the temperature-dependent unit cell volume of the average tetragonal crystallographic structure at a temperature coinciding with the onset of ferromagnetic order. We also observed the existence of a well-defined local orthorhombic structure on a short length scale of ≲5Å, resulting in a rather asymmetrical local environment of the Mn and As ions. Finally, the magnetic PDF revealed ferromagnetic alignment of Mn spins along the crystallographic c axis, with robust nearest-neighbor ferromagnetic correlations that exist even above the ferromagnetic ordering temperature. We discuss these results in the context of other experiments and theoretical studies on this system. |
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| 700 | 1 | _ | |a Billinge, Simon J. L. |0 P:(DE-HGF)0 |b 8 |
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