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000820373 1001_ $$00000-0002-7113-9769$$aHodnik, Nejc$$b0$$eCorresponding author
000820373 245__ $$aPlatinum recycling going green via induced surface potential alteration enabling fast and efficient dissolution
000820373 260__ $$aLondon$$bNature Publishing Group$$c2016
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000820373 520__ $$aThe recycling of precious metals, for example, platinum, is an essential aspect of sustainability for the modern industry and energy sectors. However, due to its resistance to corrosion, platinum-leaching techniques rely on high reagent consumption and hazardous processes, for example, boiling aqua regia; a mixture of concentrated nitric and hydrochloric acid. Here we demonstrate that complete dissolution of metallic platinum can be achieved by induced surface potential alteration, an ‘electrode-less’ process utilizing alternatively oxidative and reductive gases. This concept for platinum recycling exploits the so-called transient dissolution mechanism, triggered by a repetitive change in platinum surface oxidation state, without using any external electric current or electrodes. The effective performance in non-toxic low-concentrated acid and at room temperature is a strong benefit of this approach, potentially rendering recycling of industrial catalysts, including but not limited to platinum-based systems, more sustainable.
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000820373 7001_ $$0P:(DE-Juel1)168569$$aBaldizzone, Claudio$$b1
000820373 7001_ $$0P:(DE-HGF)0$$aPolymeros, George$$b2
000820373 7001_ $$0P:(DE-HGF)0$$aGeiger, Simon$$b3
000820373 7001_ $$0P:(DE-HGF)0$$aGrote, Jan-Philipp$$b4
000820373 7001_ $$0P:(DE-Juel1)168567$$aCherevko, Serhiy$$b5$$ufzj
000820373 7001_ $$0P:(DE-HGF)0$$aMingers, Andrea$$b6
000820373 7001_ $$0P:(DE-Juel1)168570$$aZeradjanin, Aleksandar$$b7$$ufzj
000820373 7001_ $$0P:(DE-Juel1)168125$$aMayrhofer, Karl$$b8$$eCorresponding author$$ufzj
000820373 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/ncomms13164$$gVol. 7, p. 13164 -$$p13164 -$$tNature Communications$$v7$$x2041-1723$$y2016
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