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@ARTICLE{Zhou:820894,
      author       = {Zhou, Dan and Thiele-Bruhn, Sören and Arenz-Leufen,
                      Martina Gesine and Jacques, Diederik and Lichtner, Peter and
                      Engelhardt, Irina},
      title        = {{I}mpact of manure-related {DOM} on sulfonamide transport
                      in arable soils},
      journal      = {Journal of contaminant hydrology},
      volume       = {192},
      issn         = {0169-7722},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier Science},
      reportid     = {FZJ-2016-06158},
      pages        = {118 - 128},
      year         = {2016},
      abstract     = {Field application of livestock manure introduces colloids
                      and veterinary antibiotics, e.g. sulfonamides (SAs), into
                      farmland. The presence of manure colloids may potentially
                      intensify the SAs-pollution to soils and groundwater by
                      colloid-facilitated transport. Transport of three SAs,
                      sulfadiazine (SDZ), sulfamethoxypyridazine (SMPD), and
                      sulfamoxole (SMOX), was investigated in saturated soil
                      columns with and without manure colloids from sows and
                      farrows, weaners, and fattening pigs. Experimental results
                      showed that colloid-facilitated transport of SMOX was
                      significant in the presence of manure colloids from
                      fattening pigs with low C/N ratio, high SUVA280 nm and
                      protein C, while manure colloids from sows and farrows and
                      weaners had little effect on SMOX transport. In contrast,
                      only retardation was observed for SDZ and SMPD when manure
                      colloids were present. Breakthrough curves (BTCs) of
                      colloids and SAs were replicated well by a newly developed
                      numerical model that considers colloid-filtration theory,
                      competitive kinetic sorption, and co-transport processes.
                      Model results demonstrate that mobile colloids act as
                      carriers for SMOX, while immobile colloids block SMOX from
                      sorbing onto the soil. The low affinity of SMOX to sorb on
                      immobile colloids prevents aggregation and also promotes
                      SMOX's colloid-facilitated transport. Conversely, the high
                      affinity of SDZ and SMPD to sorb on all types of immobile
                      colloids retarded their transport. Thus, manure properties
                      play a fundamental role in increasing the leaching risk of
                      hydrophobic sulfonamides.},
      cin          = {IBG-3},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IBG-3-20101118},
      pnm          = {255 - Terrestrial Systems: From Observation to Prediction
                      (POF3-255)},
      pid          = {G:(DE-HGF)POF3-255},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000383299400008},
      doi          = {10.1016/j.jconhyd.2016.07.005},
      url          = {https://juser.fz-juelich.de/record/820894},
}