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@INPROCEEDINGS{Tang:823972,
author = {Tang, Hu and Stiakakis, Emmanuel and Lettinga, M.P. and
Dhont, Jan K.G.},
title = {{S}uppressed shear banding in entangled {DNA} solution by
attractive interaction},
reportid = {FZJ-2016-06598},
year = {2016},
abstract = {Shear banding, or strain localization, a narrow zone of
intense shearing strain caused by non-homogeneous
deformation, is quite ubiquitous in solid and complex
fluids. In complex fluids, the existing of shear banding
would make conventional rheology difficult to interpret.
Especially, in entangled polymer system, the existence of
shear banding would overturn the well-known Tube theory. So
there is considerable debate over whether shear banding
observed in entangled polymers such as Polybutadiene is true
or not.We report here just by tuning the attractive
interaction between chains, the flow behaviour changes from
well-defined banded flow to almost linear flow for the same
entangled polymer system. The attractive interaction between
polymer chains is gained by grafting short PNIPA (Mw=3k)
chains on the DNA main chains with rather low grafting
density. The grafting PNIPA doesn’t change the flow
behavior of DNA at temperature lower than its LCST while at
higher temperature than LCST, the PNIPA undergoes
coil-to-globule conformation change and add an attractive
interaction on the main DNA chain, which becomes stronger
and stronger with temperature. With stronger attractive
interaction, the velocity profile becomes almost linear.
These observations would help us to understand the mechanism
for shear banding in entangle polymer systems on a molecular
level and explain why shear banding occurs in some system
but not in others.},
month = {Sep},
date = {2016-09-04},
organization = {The 30th Conference of European
Colloid and Interface Society, Rome
(Italy), 4 Sep 2016 - 9 Sep 2016},
subtyp = {After Call},
cin = {ICS-3},
cid = {I:(DE-Juel1)ICS-3-20110106},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/823972},
}