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@ARTICLE{Kampman:824282,
      author       = {Kampman, N. and Busch, A. and Bertier, P. and Snippe, J.
                      and Hangx, S. and Pipich, V. and Di, Z. and Rother, G. and
                      Harrington, J. F. and Evans, J. P. and Maskell, A. and
                      Chapman, H. J. and Bickle, M. J.},
      title        = {{O}bservational evidence confirms modelling of the
                      long-term integrity of {CO}2-reservoir caprocks},
      journal      = {Nature Communications},
      volume       = {7},
      issn         = {2041-1723},
      address      = {London},
      publisher    = {Nature Publishing Group},
      reportid     = {FZJ-2016-06901},
      pages        = {12268 -},
      year         = {2016},
      abstract     = {Storage of anthropogenic CO2 in geological formations
                      relies on a caprock as the primary seal preventing buoyant
                      super-critical CO2 escaping. Although natural CO2 reservoirs
                      demonstrate that CO2 may be stored safely for millions of
                      years, uncertainty remains in predicting how caprocks will
                      react with CO2-bearing brines. This uncertainty poses a
                      significant challenge to the risk assessment of geological
                      carbon storage. Here we describe mineral reaction fronts in
                      a CO2 reservoir-caprock system exposed to CO2 over a
                      timescale comparable with that needed for geological carbon
                      storage. The propagation of the reaction front is retarded
                      by redox-sensitive mineral dissolution reactions and
                      carbonate precipitation, which reduces its penetration into
                      the caprock to ∼7 cm in ∼105 years. This distance is
                      an order-of-magnitude smaller than previous predictions. The
                      results attest to the significance of transport-limited
                      reactions to the long-term integrity of sealing behaviour in
                      caprocks exposed to CO2.},
      cin          = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
                      (München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1 /
                      ICS-1},
      ddc          = {500},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)ICS-1-20110106},
      pnm          = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
                      Neutron Research (JCNS) (POF3-623)},
      pid          = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
      experiment   = {EXP:(DE-MLZ)KWS1-20140101 / EXP:(DE-MLZ)KWS3-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000380536100001},
      pubmed       = {pmid:27464840},
      doi          = {10.1038/ncomms12268},
      url          = {https://juser.fz-juelich.de/record/824282},
}