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@ARTICLE{Chatterji:824329,
author = {Chatterji, T. and Meven, M. and Brown, P. J.},
title = {{T}emperature evolution of magnetic structure of
{H}o{F}e{O}$_3$ by single crystal neutron diffraction},
reportid = {FZJ-2016-06938},
year = {2016},
abstract = {We have investigated the temperature evolution of the
magnetic structures of HoFeO$_3$ by single crystal neutron
diffraction. The three different magnetic structures found
as a function of temperature for \hfo\ are described by the
magnetic groups Pb$2_1$, Pbn$2_1$ and Pbn$2_1$ and are
stable in the temperature ranges $\approx$ 600-55~K, 55-37~K
and 35$>T>2$~K respectively. In all three the fundamental
coupling between the Fe sub-lattices remains the same and
only their orientation and the degree of canting away from
the ideal axial direction varies. The magnetic polarisation
of the Ho sub-lattices in these two higher temperature
regions, in which the major components of the Fe moment lie
along $x$ and $y$, is very small. The canting of the moments
from the axial directions is attributed to the antisymmetric
interactions allowed by the crystal symmetry. They include
contributions from single ion anisotropy as well as the
Dzyaloshinski antisymmetric exchange. In the low temperature
phase two further structural transitions are apparent in
which the spontaneous magnetisation changes sign with
respect to the underlying antiferromagnetic configuration.
In this temperature range the antisymmetric exchange energy
varies rapidly as the the Ho sub-lattices begin to order. So
long as the ordered Ho moments are small the antisymmetric
exchange is due only to Fe-Fe interactions, but as the
degree of Ho order increases the Fe-Ho interactions take
over whilst at the lowest temperatures, when the Ho moments
approach saturation the Ho-Ho interactions dominate. The
reversals of the spontaneous magnetisation found in this
study suggest that in \hfo\ the sums of the Fe-Fe and Ho-Ho
antisymmetric interactions have the same sign as one
another, but that of the Ho-Fe terms is opposite.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / JCNS-2},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6G15 - FRM II / MLZ (POF3-6G15) / 6212 - Quantum Condensed
Matter: Magnetism, Superconductivity (POF3-621)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15 /
G:(DE-HGF)POF3-6212},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)25},
eprint = {1604.08349},
howpublished = {arXiv:1604.08349},
archivePrefix = {arXiv},
SLACcitation = {$\%\%CITATION$ = $arXiv:1604.08349;\%\%$},
url = {https://juser.fz-juelich.de/record/824329},
}