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@ARTICLE{GarciaFresnillo:824680,
author = {Garcia-Fresnillo, L. and Patel, R. and Niewolak, Leszek and
Quadakkers, W. J. and Hua, M. and Wang, Q. and Meier, G. H.},
title = {{O}xidation {B}ehaviour and {P}hase {T}ransformations of an
{I}nterconnect {M}aterial in {S}imulated {A}node
{E}nvironment of {I}ntermediate {T}emperature {S}olid
{O}xide {F}uel {C}ells},
journal = {Materials at high temperatures},
volume = {34},
number = {1},
issn = {1878-6413},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2016-07238},
pages = {61 - 77},
year = {2016},
abstract = {The oxidation behaviour and the phase transformations
associated with high temperature exposure of a commercial
ferritic interconnect steel, Crofer 22 H, was studied in a
simulated solid oxide fuel cell (SOFC) anode atmosphere at
700 °C. Special emphasis was placed on the formation of the
intermetallic sigma phase. No sigma phase was detected in
the bulk alloy after 500 h of exposure of bare specimens.
However, specimens which were pre-coated with a layer of
nickel showed formation of an interdiffusion zone after as
little as 2 h of exposure and sigma phase formation occurred
after 10 h. The presence of the nickel layer, which
simulates the contact between ferritic steel interconnects
and a nickel mesh in a SOFC results in the formation of an
austenitic zone and accelerated formation of a σ-phase rich
layer at the ferrite/austenite interface. The ferritic steel
is transformed into austenite due to the inward diffusion of
nickel, σ-phase started to nucleate at the transformed
austenite grain boundaries. The nucleation is enhanced by an
increased Cr/Fe-ratio at that interface due to more
pronounced diffusion of Fe, compared to Cr, in the direction
of the Ni-layer. Different possible mechanisms for the
nucleation and growth of σ-phase were identified. The
experimental results led to the conclusion that sigma
nucleates in the austenite and grows following an isothermal
eutectoid-like decomposition.},
cin = {IEK-2},
ddc = {620},
cid = {I:(DE-Juel1)IEK-2-20101013},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000389473300008},
doi = {10.1080/09603409.2016.1244373},
url = {https://juser.fz-juelich.de/record/824680},
}