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@ARTICLE{Kremser:824780,
author = {Kremser, Stefanie and Thomason, Larry W. and von Hobe, Marc
and Hermann, Markus and Deshler, Terry and Timmreck, Claudia
and Toohey, Matthew and Stenke, Andrea and Schwarz, Joshua
P. and Weigel, Ralf and Fueglistaler, Stephan and Prata,
Fred J. and Vernier, Jean-Paul and Schlager, Hans and
Barnes, John E. and Antuña-Marrero, Juan-Carlos and
Fairlie, Duncan and Palm, Mathias and Mahieu, Emmanuel and
Notholt, Justus and Rex, Markus and Bingen, Christine and
Vanhellemont, Filip and Bourassa, Adam and Plane, John M. C.
and Klocke, Daniel and Carn, Simon A. and Clarisse, Lieven
and Trickl, Thomas and Neely, Ryan and James, Alexander D.
and Rieger, Landon and Wilson, James C. and Meland, Brian},
title = {{S}tratospheric aerosol-{O}bservations, processes, and
impact on climate},
journal = {Reviews of geophysics},
volume = {54},
number = {2},
issn = {8755-1209},
address = {Hoboken, NJ},
publisher = {Wiley},
reportid = {FZJ-2016-07335},
pages = {278 - 335},
year = {2016},
abstract = {Interest in stratospheric aerosol and its role in climate
have increased over the last decade due to the observed
increase in stratospheric aerosol since 2000 and the
potential for changes in the sulfur cycle induced by climate
change. This review provides an overview about the advances
in stratospheric aerosol research since the last
comprehensive assessment of stratospheric aerosol was
published in 2006. A crucial development since 2006 is the
substantial improvement in the agreement between in situ and
space-based inferences of stratospheric aerosol properties
during volcanically quiescent periods. Furthermore, new
measurement systems and techniques, both in situ and space
based, have been developed for measuring physical aerosol
properties with greater accuracy and for characterizing
aerosol composition. However, these changes induce
challenges to constructing a long-term stratospheric aerosol
climatology. Currently, changes in stratospheric aerosol
levels less than $20\%$ cannot be confidently quantified.
The volcanic signals tend to mask any nonvolcanically driven
change, making them difficult to understand. While the role
of carbonyl sulfide as a substantial and relatively constant
source of stratospheric sulfur has been confirmed by new
observations and model simulations, large uncertainties
remain with respect to the contribution from anthropogenic
sulfur dioxide emissions. New evidence has been provided
that stratospheric aerosol can also contain small amounts of
nonsulfate matter such as black carbon and organics.
Chemistry-climate models have substantially increased in
quantity and sophistication. In many models the
implementation of stratospheric aerosol processes is coupled
to radiation and/or stratospheric chemistry modules to
account for relevant feedback processes.},
cin = {IEK-7},
ddc = {550},
cid = {I:(DE-Juel1)IEK-7-20101013},
pnm = {244 - Composition and dynamics of the upper troposphere and
middle atmosphere (POF3-244)},
pid = {G:(DE-HGF)POF3-244},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000385716900002},
doi = {10.1002/2015RG000511},
url = {https://juser.fz-juelich.de/record/824780},
}