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@ARTICLE{Scheck:824899,
      author       = {Scheck, Johanna and Wu, Baohu and Drechsler, Markus and
                      Rosenberg, Rose and Van Driessche, Alexander E. S. and
                      Stawski, Tomasz M. and Gebauer, Denis},
      title        = {{T}he {M}olecular {M}echanism of {I}ron({III}) {O}xide
                      {N}ucleation},
      journal      = {The journal of physical chemistry letters},
      volume       = {7},
      number       = {16},
      issn         = {1948-7185},
      address      = {Washington, DC},
      publisher    = {ACS},
      reportid     = {FZJ-2016-07401},
      pages        = {3123 - 3130},
      year         = {2016},
      abstract     = {A molecular understanding of the formation of solid phases
                      from solution would be beneficial for various scientific
                      fields. However, nucleation pathways are still not fully
                      understood, whereby the case of iron (oxyhydr)oxides poses a
                      prime example. We show that in the prenucleation regime,
                      thermodynamically stable solute species up to a few
                      nanometers in size are observed, which meet the definition
                      of prenucleation clusters. Nucleation then is not governed
                      by a critical size, but rather by the dynamics of the
                      clusters that are forming at the distinct nucleation stages,
                      based on the chemistry of the linkages within the clusters.
                      This resolves a longstanding debate in the field of iron
                      oxide nucleation, and the results may generally apply to
                      oxides forming via hydrolysis and condensation. The
                      (molecular) understanding of the chemical basis of phase
                      separation is paramount for, e.g., tailoring size, shape and
                      structure of novel nanocrystalline materials.},
      cin          = {ICS-1 / Neutronenstreuung ; JCNS-1 / JCNS (München) ;
                      Jülich Centre for Neutron Science JCNS (München) ;
                      JCNS-FRM-II},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106 /
                      I:(DE-Juel1)JCNS-FRM-II-20110218},
      pnm          = {551 - Functional Macromolecules and Complexes (POF3-551) /
                      6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6215 - Soft Matter, Health and Life Sciences (POF3-621)},
      pid          = {G:(DE-HGF)POF3-551 / G:(DE-HGF)POF3-6G4 /
                      G:(DE-HGF)POF3-6215},
      experiment   = {EXP:(DE-MLZ)NOSPEC-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000381781800010},
      pubmed       = {pmid:27466739},
      doi          = {10.1021/acs.jpclett.6b01237},
      url          = {https://juser.fz-juelich.de/record/824899},
}