000824950 001__ 824950
000824950 005__ 20240619092027.0
000824950 0247_ $$2doi$$a10.1038/srep35034
000824950 0247_ $$2Handle$$a2128/13201
000824950 0247_ $$2WOS$$aWOS:000385063300001
000824950 0247_ $$2altmetric$$aaltmetric:12147019
000824950 0247_ $$2pmid$$apmid:27725747
000824950 037__ $$aFZJ-2016-07446
000824950 041__ $$aEnglish
000824950 082__ $$a000
000824950 1001_ $$0P:(DE-Juel1)130679$$aGupta, S.$$b0$$eCorresponding author$$ufzj
000824950 245__ $$aEffect of adding nanometre-sized heterogeneities on the structural dynamics and the excess wing of a molecular glass former
000824950 260__ $$aLondon$$bNature Publishing Group$$c2016
000824950 3367_ $$2DRIVER$$aarticle
000824950 3367_ $$2DataCite$$aOutput Types/Journal article
000824950 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1481640465_20885
000824950 3367_ $$2BibTeX$$aARTICLE
000824950 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000824950 3367_ $$00$$2EndNote$$aJournal Article
000824950 520__ $$aWe present the relaxation dynamics of glass-forming glycerol mixed with 1.1 nm sized polyhedral oligomeric silsesquioxane (POSS) molecules using dielectric spectroscopy (DS) and two different neutron scattering (NS) techniques. Both, the reorientational dynamics as measured by DS and the density fluctuations detected by NS reveal a broadening of the α relaxation when POSS molecules are added. Moreover, we find a significant slowing down of the α-relaxation time. These effects are in accord with the heterogeneity scenario considered for the dynamics of glasses and supercooled liquids. The addition of POSS also affects the excess wing in glycerol arising from a secondary relaxation process, which seems to exhibit a dramatic increase in relative strength compared to the α relaxation.
000824950 536__ $$0G:(DE-HGF)POF3-551$$a551 - Functional Macromolecules and Complexes (POF3-551)$$cPOF3-551$$fPOF III$$x0
000824950 536__ $$0G:(DE-HGF)POF3-6G4$$a6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)$$cPOF3-623$$fPOF III$$x1
000824950 536__ $$0G:(DE-HGF)POF3-6215$$a6215 - Soft Matter, Health and Life Sciences (POF3-621)$$cPOF3-621$$fPOF III$$x2
000824950 588__ $$aDataset connected to CrossRef
000824950 7001_ $$0P:(DE-HGF)0$$aFischer, J. K. H.$$b1
000824950 7001_ $$0P:(DE-HGF)0$$aLunkenheimer, P.$$b2
000824950 7001_ $$0P:(DE-HGF)0$$aLoidl, A.$$b3
000824950 7001_ $$0P:(DE-HGF)0$$aNovak, E.$$b4
000824950 7001_ $$0P:(DE-Juel1)143752$$aJalarvo, N.$$b5$$ufzj
000824950 7001_ $$0P:(DE-Juel1)130872$$aOhl, M.$$b6$$ufzj
000824950 773__ $$0PERI:(DE-600)2615211-3$$a10.1038/srep35034$$gVol. 6, p. 35034 -$$p35034 -$$tScientific reports$$v6$$x2045-2322$$y2016
000824950 8564_ $$uhttps://juser.fz-juelich.de/record/824950/files/srep35034.pdf$$yOpenAccess
000824950 8564_ $$uhttps://juser.fz-juelich.de/record/824950/files/srep35034.gif?subformat=icon$$xicon$$yOpenAccess
000824950 8564_ $$uhttps://juser.fz-juelich.de/record/824950/files/srep35034.jpg?subformat=icon-1440$$xicon-1440$$yOpenAccess
000824950 8564_ $$uhttps://juser.fz-juelich.de/record/824950/files/srep35034.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000824950 8564_ $$uhttps://juser.fz-juelich.de/record/824950/files/srep35034.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000824950 8564_ $$uhttps://juser.fz-juelich.de/record/824950/files/srep35034.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000824950 8767_ $$8217038OI$$92016-09-28$$d2016-10-04$$eAPC$$jZahlung erfolgt$$zSREP-16-17793A
000824950 909CO $$ooai:juser.fz-juelich.de:824950$$pdnbdelivery$$popenCost$$pVDB$$pdriver$$pOpenAPC$$popen_access$$popenaire
000824950 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130679$$aForschungszentrum Jülich$$b0$$kFZJ
000824950 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)143752$$aForschungszentrum Jülich$$b5$$kFZJ
000824950 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130872$$aForschungszentrum Jülich$$b6$$kFZJ
000824950 9131_ $$0G:(DE-HGF)POF3-551$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bKey Technologies$$lBioSoft – Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vFunctional Macromolecules and Complexes$$x0
000824950 9131_ $$0G:(DE-HGF)POF3-623$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-6G4$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vFacility topic: Neutrons for Research on Condensed Matter$$x1
000824950 9131_ $$0G:(DE-HGF)POF3-621$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-6215$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vIn-house research on the structure, dynamics and function of matter$$x2
000824950 9141_ $$y2016
000824950 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000824950 915__ $$0StatID:(DE-HGF)1050$$2StatID$$aDBCoverage$$bBIOSIS Previews
000824950 915__ $$0LIC:(DE-HGF)CCBY4$$2HGFVOC$$aCreative Commons Attribution CC BY 4.0
000824950 915__ $$0StatID:(DE-HGF)1040$$2StatID$$aDBCoverage$$bZoological Record
000824950 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bSCI REP-UK : 2015
000824950 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bSCI REP-UK : 2015
000824950 915__ $$0StatID:(DE-HGF)0501$$2StatID$$aDBCoverage$$bDOAJ Seal
000824950 915__ $$0StatID:(DE-HGF)0500$$2StatID$$aDBCoverage$$bDOAJ
000824950 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000824950 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000824950 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000824950 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000824950 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000824950 915__ $$0StatID:(DE-HGF)0310$$2StatID$$aDBCoverage$$bNCBI Molecular Biology Database
000824950 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000824950 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000824950 9201_ $$0I:(DE-Juel1)ICS-1-20110106$$kICS-1$$lNeutronenstreuung $$x0
000824950 9201_ $$0I:(DE-Juel1)JCNS-1-20110106$$kNeutronenstreuung ; JCNS-1$$lNeutronenstreuung $$x1
000824950 9201_ $$0I:(DE-Juel1)JCNS-SNS-20110128$$kJCNS-SNS$$lJCNS-SNS$$x2
000824950 9801_ $$aFullTexts
000824950 980__ $$ajournal
000824950 980__ $$aVDB
000824950 980__ $$aUNRESTRICTED
000824950 980__ $$aI:(DE-Juel1)ICS-1-20110106
000824950 980__ $$aI:(DE-Juel1)JCNS-1-20110106
000824950 980__ $$aI:(DE-Juel1)JCNS-SNS-20110128
000824950 980__ $$aAPC
000824950 981__ $$aI:(DE-Juel1)IBI-8-20200312
000824950 981__ $$aI:(DE-Juel1)JCNS-1-20110106
000824950 981__ $$aI:(DE-Juel1)JCNS-1-20110106
000824950 981__ $$aI:(DE-Juel1)JCNS-SNS-20110128