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@ARTICLE{Thalinger:825375,
      author       = {Thalinger, Ramona and Gocyla, Martin and Heggen, Marc and
                      Dunin-Borkowski, Rafal and Grünbacher, Matthias and
                      Stöger-Pollach, Michael and Schmidmair, Daniela and
                      Klötzer, Bernhard and Penner, Simon},
      title        = {{N}i–perovskite interaction and its structural and
                      catalytic consequences in methane steam reforming and
                      methanation reactions},
      journal      = {Journal of catalysis},
      volume       = {337},
      issn         = {0021-9517},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2016-07838},
      pages        = {26 - 35},
      year         = {2016},
      abstract     = {Metal–support interaction effects and their consequences
                      in CO2/CO methanation and methane steam reforming have been
                      exemplarily studied on two complex Ni–perovskite powder
                      catalyst systems, namely Ni–La0.6Sr0.4FeO3−δ (lanthanum
                      strontium ferrite, LSF) and Ni–SrTi0.7Fe0.3O3−δ
                      (strontium titanium ferrite, STF). Pre-reduction in hydrogen
                      and treatment in catalytic gas mixtures cause a variety of
                      structural effects, including exsolution of iron particles
                      and formation of Ni–Fe alloy particles. These
                      manifestations strongly depend on the reducibility of the
                      perovskite and are hence much more pronounced on LSF.
                      Reactivity differences are strongly influenced by the
                      chemical properties of the respective perovskite support.
                      The more reducible the perovskite support, the stronger the
                      deviation from the catalytic behavior of a Ni/Al2O3
                      reference catalyst, rendering establishments of direct
                      structure–activity/selectivity relationships difficult.
                      The studies show the extreme variety of the
                      metal–perovskite interface, which helps in judging similar
                      systems of recent high catalytic importance, e.g. metals
                      supported on spinel or other perovskite phases.},
      cin          = {PGI-5},
      ddc          = {540},
      cid          = {I:(DE-Juel1)PGI-5-20110106},
      pnm          = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
      pid          = {G:(DE-HGF)POF3-143},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000374920400003},
      doi          = {10.1016/j.jcat.2016.01.020},
      url          = {https://juser.fz-juelich.de/record/825375},
}