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@ARTICLE{Schraknepper:826225,
      author       = {Schraknepper, H. and Bäumer, C. and Gunkel, F. and
                      Dittmann, R. and De Souza, R. A.},
      title        = {{P}ulsed laser deposition of {S}r{R}u{O} 3 thin-films:
                      {T}he role of the pulse repetition rate},
      journal      = {APL materials},
      volume       = {4},
      number       = {12},
      issn         = {2166-532X},
      address      = {Melville, NY},
      publisher    = {AIP Publ.},
      reportid     = {FZJ-2017-00471},
      pages        = {126109 -},
      year         = {2016},
      abstract     = {SrRuO3 thin-films were deposited with different pulse
                      repetition rates, fdep, epitaxially on vicinal SrTiO3
                      substrates by means of pulsed laser deposition. The
                      measurement of several physical properties (e.g.,
                      composition by means of X-ray photoelectron spectroscopy,
                      the out-of-plane lattice parameter, the electric
                      conductivity, and the Curie temperature) consistently
                      reveals that an increase in laser repetition rate results in
                      an increase in ruthenium deficiency in the films. By the
                      same token, it is shown that when using low repetition
                      rates, approaching a nearly stoichiometric cation ratio in
                      SrRuO3 becomes feasible. Based on these results, we propose
                      a mechanism to explain the widely observed Ru deficiency of
                      SrRuO3 thin-films. Our findings demand these theoretical
                      considerations to be based on kinetic rather than widely
                      employed thermodynamic arguments.},
      cin          = {PGI-7},
      ddc          = {620},
      cid          = {I:(DE-Juel1)PGI-7-20110106},
      pnm          = {521 - Controlling Electron Charge-Based Phenomena
                      (POF3-521)},
      pid          = {G:(DE-HGF)POF3-521},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000391991100010},
      doi          = {10.1063/1.4972996},
      url          = {https://juser.fz-juelich.de/record/826225},
}