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@ARTICLE{Willenbockel:826503,
      author       = {Willenbockel, Martin and Maurer, Reinhard J. and Bronner,
                      Christopher and Schulze, Michael and Stadtmüller, Benjamin
                      and Soubatch, Serguei and Tegeder, Petra and Reuter, Karsten
                      and Tautz, Frank Stefan},
      title        = {{C}overage-driven dissociation of azobenzene on {C}u(111):
                      a route towards defined surface functionalization},
      journal      = {Chemical communications},
      volume       = {51},
      number       = {83},
      issn         = {1364-548X},
      address      = {Cambridge},
      publisher    = {Soc.},
      reportid     = {FZJ-2017-00726},
      pages        = {15324 - 15327},
      year         = {2015},
      abstract     = {We investigate the surface-catalyzed dissociation of the
                      archetypal molecular switch azobenzene on the Cu(111)
                      surface. Based on X-ray photoelectron spectroscopy, normal
                      incidence X-ray standing waves and density functional theory
                      calculations a detailed picture of the coverage-induced
                      formation of phenyl nitrene from azobenzene is presented.
                      Furthermore, a comparison to the azobenzene/Ag(111)
                      interface provides insight into the driving force behind the
                      dissociation on Cu(111). The quantitative decay of
                      azobenzene paves the way for the creation of a defect free,
                      covalently bonded monolayer. Our work suggests a route of
                      surface functionalization via suitable azobenzene
                      derivatives and the on surface synthesis concept, allowing
                      for the creation of complex immobilized molecular systems.},
      cin          = {PGI-3 / JARA-FIT},
      ddc          = {540},
      cid          = {I:(DE-Juel1)PGI-3-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {141 - Controlling Electron Charge-Based Phenomena
                      (POF3-141)},
      pid          = {G:(DE-HGF)POF3-141},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000363167000025},
      doi          = {10.1039/C5CC05003K},
      url          = {https://juser.fz-juelich.de/record/826503},
}