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| Hauptseite > Publikationsdatenbank > Coverage-driven dissociation of azobenzene on Cu(111): a route towards defined surface functionalization > print |
| Hauptseite > Publikationsdatenbank > Coverage-driven dissociation of azobenzene on Cu(111): a route towards defined surface functionalization > print |
| 001 | 826503 | ||
| 005 | 20210129225629.0 | ||
| 024 | 7 | _ | |a 10.1039/C5CC05003K |2 doi |
| 024 | 7 | _ | |a 0009-241X |2 ISSN |
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| 024 | 7 | _ | |a 1359-7345 |2 ISSN |
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| 100 | 1 | _ | |a Willenbockel, Martin |0 P:(DE-Juel1)142384 |b 0 |
| 245 | _ | _ | |a Coverage-driven dissociation of azobenzene on Cu(111): a route towards defined surface functionalization |
| 260 | _ | _ | |a Cambridge |c 2015 |b Soc. |
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| 520 | _ | _ | |a We investigate the surface-catalyzed dissociation of the archetypal molecular switch azobenzene on the Cu(111) surface. Based on X-ray photoelectron spectroscopy, normal incidence X-ray standing waves and density functional theory calculations a detailed picture of the coverage-induced formation of phenyl nitrene from azobenzene is presented. Furthermore, a comparison to the azobenzene/Ag(111) interface provides insight into the driving force behind the dissociation on Cu(111). The quantitative decay of azobenzene paves the way for the creation of a defect free, covalently bonded monolayer. Our work suggests a route of surface functionalization via suitable azobenzene derivatives and the on surface synthesis concept, allowing for the creation of complex immobilized molecular systems. |
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| 700 | 1 | _ | |a Maurer, Reinhard J. |0 P:(DE-HGF)0 |b 1 |
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| 700 | 1 | _ | |a Stadtmüller, Benjamin |0 P:(DE-Juel1)139025 |b 4 |
| 700 | 1 | _ | |a Soubatch, Serguei |0 P:(DE-HGF)0 |b 5 |e Corresponding author |
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| 773 | _ | _ | |a 10.1039/C5CC05003K |g Vol. 51, no. 83, p. 15324 - 15327 |0 PERI:(DE-600)1472881-3 |n 83 |p 15324 - 15327 |t Chemical communications |v 51 |y 2015 |x 1364-548X |
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