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000827075 245__ $$aSpiral spin-liquid and the emergence of a vortex-like state in MnSc2S4
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000827075 520__ $$aSpirals and helices are common motifs of long-range order in magnetic solids, and they may also be organized into more complex emergent structures such as magnetic skyrmions and vortices. A new type of spiral state, the spiral spin-liquid, in which spins fluctuate collectively as spirals, has recently been predicted to exist. Here, using neutron scattering techniques, we experimentally prove the existence of a spiral spin-liquid in MnSc2S4 by directly observing the ‘spiral surface’—a continuous surface of spiral propagation vectors in reciprocal space. We elucidate the multi-step ordering behaviour of the spiral spin-liquid, and discover a vortex-like triple-q phase on application of a magnetic field. Our results prove the effectiveness of the J1–J2 Hamiltonian on the diamond lattice as a model for the spiral spin-liquid state in MnSc2S4, and also demonstrate a new way to realize a magnetic vortex lattice through frustrated interactions.
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000827075 65017 $$0V:(DE-MLZ)GC-1604-2016$$2V:(DE-HGF)$$aMagnetic Materials$$x0
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000827075 7001_ $$0P:(DE-HGF)0$$aZaharko, Oksana$$b1$$eCorresponding author
000827075 7001_ $$0P:(DE-HGF)0$$aTsurkan, Vladimir$$b2
000827075 7001_ $$0P:(DE-Juel1)130991$$aSu, Yixi$$b3
000827075 7001_ $$0P:(DE-HGF)0$$aWhite, Jonathan S.$$b4
000827075 7001_ $$0P:(DE-HGF)0$$aTucker, Gregory S.$$b5
000827075 7001_ $$0P:(DE-HGF)0$$aRoessli, Bertrand$$b6
000827075 7001_ $$0P:(DE-HGF)0$$aBourdarot, Frederic$$b7
000827075 7001_ $$0P:(DE-HGF)0$$aSibille, Romain$$b8
000827075 7001_ $$0P:(DE-HGF)0$$aChernyshov, Dmitry$$b9
000827075 7001_ $$0P:(DE-HGF)0$$aFennell, Tom$$b10
000827075 7001_ $$0P:(DE-HGF)0$$aLoidl, Alois$$b11
000827075 7001_ $$0P:(DE-HGF)0$$aRüegg, Christian$$b12
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