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100 1 _ |a Gao, Shang
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245 _ _ |a Spiral spin-liquid and the emergence of a vortex-like state in MnSc2S4
260 _ _ |a Basingstoke
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520 _ _ |a Spirals and helices are common motifs of long-range order in magnetic solids, and they may also be organized into more complex emergent structures such as magnetic skyrmions and vortices. A new type of spiral state, the spiral spin-liquid, in which spins fluctuate collectively as spirals, has recently been predicted to exist. Here, using neutron scattering techniques, we experimentally prove the existence of a spiral spin-liquid in MnSc2S4 by directly observing the ‘spiral surface’—a continuous surface of spiral propagation vectors in reciprocal space. We elucidate the multi-step ordering behaviour of the spiral spin-liquid, and discover a vortex-like triple-q phase on application of a magnetic field. Our results prove the effectiveness of the J1–J2 Hamiltonian on the diamond lattice as a model for the spiral spin-liquid state in MnSc2S4, and also demonstrate a new way to realize a magnetic vortex lattice through frustrated interactions.
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693 _ _ |a Forschungs-Neutronenquelle Heinz Maier-Leibnitz
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700 1 _ |a Zaharko, Oksana
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700 1 _ |a Tsurkan, Vladimir
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700 1 _ |a Su, Yixi
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700 1 _ |a White, Jonathan S.
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700 1 _ |a Tucker, Gregory S.
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700 1 _ |a Roessli, Bertrand
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700 1 _ |a Bourdarot, Frederic
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700 1 _ |a Sibille, Romain
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700 1 _ |a Chernyshov, Dmitry
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700 1 _ |a Fennell, Tom
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700 1 _ |a Loidl, Alois
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700 1 _ |a Rüegg, Christian
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773 _ _ |a 10.1038/nphys3914
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