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000827462 1001_ $$0P:(DE-HGF)0$$aLançon, Diane$$b0$$eCorresponding author
000827462 245__ $$aMnO nanoparticles as the cause of ferromagnetism in bulk dilute Mn-doped ZnO
000827462 260__ $$aMelville, NY$$bAmerican Inst. of Physics$$c2016
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000827462 520__ $$aWe show that the observed ferromagnetic behavior of ZnO lightly doped with Mn coincides with the presence of MnO nanoparticles, whereas cluster-free Mn doped ZnO behaves paramagnetically. This conclusion is reached by a study of the structural and magnetic properties of powdered samples of (Mnx,Zn1–x)O with x ≤ 0.033 using polarized neutron scattering. Two types of samples were synthesized via, respectively, a solid state method and the decomposition of hydrozincite. Further characterization has been performed using standard X-ray diffraction and magnetization measurements. The results show evidence for the formation of MnO nanoparticles in the highest doped samples for both synthesis methods, with a ferromagnetic behavior attributed to uncompensated Mn2+ in the MnO nanoparticles. The lower Mn-doped samples showed no evidence for structural segregation or magnetic correlations and showed only a paramagnetic behaviour.
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000827462 7001_ $$0P:(DE-HGF)0$$aNilsen, Gøran J.$$b1
000827462 7001_ $$0P:(DE-HGF)0$$aWildes, Andrew R.$$b2
000827462 7001_ $$0P:(DE-Juel1)141702$$aNemkovski, Kirill$$b3
000827462 7001_ $$0P:(DE-HGF)0$$aHuang, Ping$$b4
000827462 7001_ $$0P:(DE-HGF)0$$aFejes, Dóra$$b5
000827462 7001_ $$00000-0002-8832-8865$$aRønnow, Henrik M.$$b6
000827462 7001_ $$0P:(DE-HGF)0$$aMagrez, Arnaud$$b7
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