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@ARTICLE{Eiteneer:827778,
author = {Eiteneer, D. and Pálsson, G. K. and Nemšák, S. and Gray,
A. X. and Kaiser, A. M. and Son, J. and LeBeau, J. and
Conti, G. and Greer, A. A. and Keqi, A. and Rattanachata, A.
and Saw, A. Y. and Bostwick, A. and Rotenberg, E. and
Gullikson, E. M. and Ueda, S. and Kobayashi, K. and Janotti,
A. and Van de Walle, C. G. and Blanca-Romero, A. and
Pentcheva, R. and Schneider, C. M. and Stemmer, S. and
Fadley, C. S.},
title = {{D}epth-{R}esolved {C}omposition and {E}lectronic
{S}tructure of {B}uried {L}ayers and {I}nterfaces in a
{L}a{N}i{O}$_{3}$/{S}r{T}i{O}$_{3}$ {S}uperlattice from
{S}oft- and {H}ard- {X}-ray {S}tanding-{W}ave
{A}ngle-{R}esolved {P}hotoemission},
journal = {Journal of electron spectroscopy and related phenomena},
volume = {211},
issn = {0368-2048},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2017-01882},
pages = {70 - 81},
year = {2016},
abstract = {LaNiO3 (LNO) is an intriguing member of the rare-earth
nickelates in exhibiting a metal-insulator transition for a
critical film thickness of about 4 unit cells [Son et al.,
Appl. Phys. Lett. 96, 062114 (2010)]; however, such thin
films also show a transition to a metallic state in
superlattices with SrTiO3 (STO) [Son et al., Appl. Phys.
Lett. 97, 202109 (2010)]. In order to better understand this
transition, we have studied a strained LNO/STO superlattice
with 10 repeats of [4 unit-cell LNO/3 unit-cell STO] grown
on an (LaAlO3)0.3(Sr2AlTaO6)0.7 substrate using soft x-ray
standing-wave-excited angle-resolved photoemission
(SWARPES), together with soft- and hard- x-ray photoemission
measurements of core levels and densities-of-states valence
spectra. The experimental results are compared with
state-of-the-art density functional theory (DFT)
calculations of band structures and densities of states.
Using core-level rocking curves and x-ray optical modeling
to assess the position of the standing wave, SWARPES
measurements are carried out for various incidence angles
and used to determine interface-specific changes in
momentum-resolved electronic structure. We further show that
the momentum-resolved behavior of the Ni 3d eg and t2g
states near the Fermi level, as well as those at the bottom
of the valence bands, is very similar to recently published
SWARPES results for a related La0.7Sr0.3MnO3/SrTiO3
superlattice that was studied using the same technique (Gray
et al., Europhysics Letters 104, 17004 (2013)), which
further validates this experimental approach and our
conclusions. Our conclusions are also supported in several
ways by comparison to DFT calculations for the parent
materials and the superlattice, including layer-resolved
density-of-states results.},
cin = {PGI-6},
ddc = {620},
cid = {I:(DE-Juel1)PGI-6-20110106},
pnm = {522 - Controlling Spin-Based Phenomena (POF3-522)},
pid = {G:(DE-HGF)POF3-522},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000382343100009},
doi = {10.1016/j.elspec.2016.04.008},
url = {https://juser.fz-juelich.de/record/827778},
}