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@ARTICLE{Nemk:827779,
author = {Nemšák, S. and Conti, G. and Gray, A. X. and Palsson, G.
K. and Conlon, C. and Eiteneer, D. and Keqi, A. and
Rattanachata, A. and Saw, A. Y. and Bostwick, A. and
Moreschini, L. and Rotenberg, E. and Strocov, V. N. and
Kobayashi, M. and Schmitt, T. and Stolte, W. and Ueda, S.
and Kobayashi, K. and Gloskovskii, A. and Drube, W. and
Jackson, C. A. and Moetakef, P. and Janotti, A. and Bjaalie,
L. and Himmetoglu, B. and Van de Walle, C. G. and Borek, S.
and Minar, J. and Braun, J. and Ebert, H. and Plucinski, L.
and Kortright, J. B. and Schneider, C. M. and Balents, L.
and de Groot, F. M. F. and Stemmer, S. and Fadley, C. S.},
title = {{E}nergetic, spatial, and momentum character of the
electronic structure at a buried interface: {T}he
two-dimensional electron gas between two metal oxides},
journal = {Physical review / B},
volume = {93},
number = {24},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2017-01883},
pages = {245103},
year = {2016},
abstract = {The interfaces between two condensed phases often exhibit
emergent physical properties that can lead to new physics
and novel device applications and are the subject of intense
study in many disciplines. We here apply experimental and
theoretical techniques to the characterization of one such
interesting interface system: the two-dimensional electron
gas (2DEG) formed in multilayers consisting of SrTiO3 (STO)
and GdTiO3 (GTO). This system has been the subject of
multiple studies recently and shown to exhibit very high
carrier charge densities and ferromagnetic effects, among
other intriguing properties. We have studied a 2DEG-forming
multilayer of the form [6unitcells(u.c.)STO/3u.c.ofGTO]20
using a unique array of photoemission techniques including
soft and hard x-ray excitation, soft x-ray angle-resolved
photoemission, core-level spectroscopy, resonant excitation,
and standing-wave effects, as well as theoretical
calculations of the electronic structure at several levels
and of the actual photoemission process. Standing-wave
measurements below and above a strong resonance have been
exploited as a powerful method for studying the 2DEG depth
distribution. We have thus characterized the spatial and
momentum properties of this 2DEG in detail, determining via
depth-distribution measurements that it is spread throughout
the 6 u.c. layer of STO and measuring the momentum
dispersion of its states. The experimental results are
supported in several ways by theory, leading to a much more
complete picture of the nature of this 2DEG and suggesting
that oxygen vacancies are not the origin of it. Similar
multitechnique photoemission studies of such states at
buried interfaces, combined with comparable theory, will be
a very fruitful future approach for exploring and modifying
the fascinating world of buried-interface physics and
chemistry.},
cin = {PGI-6},
ddc = {530},
cid = {I:(DE-Juel1)PGI-6-20110106},
pnm = {522 - Controlling Spin-Based Phenomena (POF3-522)},
pid = {G:(DE-HGF)POF3-522},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000376996000003},
doi = {10.1103/PhysRevB.93.245103},
url = {https://juser.fz-juelich.de/record/827779},
}