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@MISC{Jiang:827862,
author = {Jiang, Xiaoqian and Klumpp, Erwin and Cade-Menun, Barbara
J. and Bol, Roland and Nischwitz, Volker and Willbold,
Sabine and Vereecken, Harry and Bauke, Sara L. and Amelung,
Wulf},
title = {{C}olloid-bound and dissolved phosphorus species in topsoil
water extracts along a grassland transect from {C}ambisol to
{S}tagnosol},
reportid = {FZJ-2017-01950},
year = {2017},
note = {Forschungsdaten zum gleichnamigen Journalartikel},
abstract = {Phosphorus (P) species in colloidal and “dissolved”
soil fractions may have different distributions. To
understand which P species are potentially involved, we
obtained water extracts from the surface soils of a gradient
5 from Cambisol, Stagnic Cambisol to Stagnosol from
temperate grassland in Germany. These were filtered to <450
nm, and divided into three procedurally defined fractions:
small-sized colloids (20–450 nm), nano-sized colloids
(1–20 nm), and “dissolved P” (<1 nm), using asymmetric
flow 10 field-flow fractionation (AF4), as well as
filtration for solution 31P-nuclear magnetic resonance (NMR)
spectroscopy. The total P of soil water extracts increased
in the order Cambisol<Stagnic Cambisol<Stagnosol due to
increasing contributions from the dissolved P fraction.
Associations of C–Fe/Al–PO3 15 4 /pyrophosphate were
absent in nanosized (1–20 nm) colloids from the Cambisol
but not in the Stagnosol. The 31P-NMR results indicated that
this was accompanied by elevated portions of organic P in
the order Cambisol>Stagnic Cambisol>Stagnosol. Across all 20
soil types, elevated proportions of inositol
hexakisphosphate (IHP) species (e.g., myo-, scyllo- and
D-chiro-IHP) were associated with soil mineral particles
(i.e., bulk soil and small-sized soil colloids), whereas
other orthophosphate monoesters and phosphonates were found
in the “dissolved” 25 P fraction. We conclude that P
species composition varies among colloidal and
“dissolved” soil fractions after characterization using
advanced techniques, i.e., AF4 and NMR. Furthermore, stagnic
properties affect P speciation and availability by
potentially releasing dissolved inorganic and esterbound P
forms as well as nano-sized organic matter–Fe/Al–P 30
colloids.},
cin = {IBG-3 / ZEA-3},
ddc = {570},
cid = {I:(DE-Juel1)IBG-3-20101118 / I:(DE-Juel1)ZEA-3-20090406},
pnm = {255 - Terrestrial Systems: From Observation to Prediction
(POF3-255)},
pid = {G:(DE-HGF)POF3-255},
typ = {PUB:(DE-HGF)32},
url = {https://juser.fz-juelich.de/record/827862},
}