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@ARTICLE{Huttmann:827875,
author = {Huttmann, Felix and Klar, David and Atodiresei, Nicolae and
Schmitz-Antoniak, Carolin and Smekhova, Alevtina and
Martínez-Galera, Antonio J. and Caciuc, Vasile and
Bihlmayer, Gustav and Blügel, Stefan and Michely, Thomas
and Wende, Heiko},
title = {{M}agnetism in a graphene- 4 f − 3 d hybrid system},
journal = {Physical review / B},
volume = {95},
number = {7},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2017-01958},
pages = {075427},
year = {2017},
abstract = {We create an interface of graphene with a metallic and
magnetic support that leaves its electronic structure
largely intact. This is achieved by exposing epitaxial
graphene on ferromagnetic thin films of Co and Ni to vapor
of the rare earth metal Eu at elevated temperatures,
resulting in the intercalation of an Eu monolayer in between
graphene and its substrate. The system is atomically well
defined, with the Eu monolayer forming a (√3×√3)R30∘
superstructure with respect to the graphene lattice.
Thereby, we avoid the strong hybridization with the (Ni,Co)
substrate 3d states that otherwise drastically modify the
electronic structure of graphene. This picture is suggested
by our x-ray absorption spectroscopy measurements which show
that after Eu intercalation the empty 2p states of C atoms
resemble more the ones measured for graphite in contrast to
graphene directly bound to 3d ferromagnetic substrates. We
use x-ray magnetic circular dichroism at the Co and Ni L2,3
and Eu M4,5 as an element-specific probe to investigate
magnetism in these systems. An antiferromagnetic coupling
between Eu and Co/Ni moments is found, which is so strong
that a magnetic moment of the Eu layer can be detected at
room temperature. Density functional theory calculations
confirm the antiferromagnetic coupling and provide an atomic
insight into the magnetic coupling mechanism.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC / PGI-6},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$ /
I:(DE-Juel1)PGI-6-20110106},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000394659700008},
doi = {10.1103/PhysRevB.95.075427},
url = {https://juser.fz-juelich.de/record/827875},
}