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000828100 1001_ $$0P:(DE-HGF)0$$avan den Ham, E. J.$$b0$$eCorresponding author
000828100 245__ $$a3D indium tin oxide electrodes by ultrasonic spray deposition for current collection applications
000828100 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2017
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000828100 520__ $$aThree dimensionally (3D) structured indium tin oxide (ITO) thin films are synthesized and characterized as a 3D electrode material for current collection applications. Using metal citrate chemistry in combination with ultrasonic spray deposition, a low cost wet-chemical method has been developed to achieve conformal ITO coatings on non-planar scaffolds. Although there is room for improvement with respect to the resistivity (9.9·10−3 Ω∙cm, 220 nm thick planar films), high quality 3D structured coatings were shown to exhibit conductive properties based on ferrocene reactivity. In view of applications in Li-ion batteries, the electrochemical stability of the current collector was investigated, indicating that stability is guaranteed for voltages of 1.5 V and up (vs. Li+/Li). In addition, subsequent 3D coating of the ITO with WO3 as a negative electrode (battery) material confirmed the 3D ITO layer functions as a proper current collector. Using this approach, an over 4-fold capacity increase was booked for 3D structured WO3 in comparison to planar samples, confirming the current collecting capabilities of the 3D ITO coating. Therefore, the 3D ITO presented is considered as a highly interesting material for 3D battery applications and beyond.
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000828100 7001_ $$0P:(DE-HGF)0$$aBonneux, G.$$b2
000828100 7001_ $$0P:(DE-HGF)0$$aMaino, G.$$b3
000828100 7001_ $$0P:(DE-Juel1)165918$$aNotten, P. H. L.$$b4$$ufzj
000828100 7001_ $$0P:(DE-HGF)0$$aVan Bael, M. K.$$b5
000828100 7001_ $$0P:(DE-HGF)0$$aHardy, A.$$b6
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