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000828162 1001_ $$0P:(DE-HGF)0$$aKourtchev, Ivan$$b0$$eCorresponding author
000828162 245__ $$aEnhanced Volatile Organic Compounds emissions and organic aerosol mass increase the oligomer content of atmospheric aerosols
000828162 260__ $$aLondon$$bNature Publishing Group$$c2016
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000828162 520__ $$aSecondary organic aerosol (SOA) accounts for a dominant fraction of the submicron atmospheric particle mass, but knowledge of the formation, composition and climate effects of SOA is incomplete and limits our understanding of overall aerosol effects in the atmosphere. Organic oligomers were discovered as dominant components in SOA over a decade ago in laboratory experiments and have since been proposed to play a dominant role in many aerosol processes. However, it remains unclear whether oligomers are relevant under ambient atmospheric conditions because they are often not clearly observed in field samples. Here we resolve this long-standing discrepancy by showing that elevated SOA mass is one of the key drivers of oligomer formation in the ambient atmosphere and laboratory experiments. We show for the first time that a specific organic compound class in aerosols, oligomers, is strongly correlated with cloud condensation nuclei (CCN) activities of SOA particles. These findings might have important implications for future climate scenarios where increased temperatures cause higher biogenic volatile organic compound (VOC) emissions, which in turn lead to higher SOA mass formation and significant changes in SOA composition. Such processes would need to be considered in climate models for a realistic representation of future aerosol-climate-biosphere feedbacks.
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000828162 7001_ $$0P:(DE-HGF)0$$aGiorio, Chiara$$b1
000828162 7001_ $$0P:(DE-HGF)0$$aManninen, Antti$$b2
000828162 7001_ $$0P:(DE-HGF)0$$aWilson, Eoin$$b3
000828162 7001_ $$0P:(DE-HGF)0$$aMahon, Brendan$$b4
000828162 7001_ $$0P:(DE-HGF)0$$aAalto, Juho$$b5
000828162 7001_ $$0P:(DE-HGF)0$$aKajos, Maija$$b6
000828162 7001_ $$0P:(DE-HGF)0$$aVenables, Dean$$b7
000828162 7001_ $$0P:(DE-HGF)0$$aRuuskanen, Taina$$b8
000828162 7001_ $$0P:(DE-HGF)0$$aLevula, Janne$$b9
000828162 7001_ $$0P:(DE-HGF)0$$aLoponen, Matti$$b10
000828162 7001_ $$0P:(DE-HGF)0$$aConnors, Sarah$$b11
000828162 7001_ $$0P:(DE-HGF)0$$aHarris, Neil$$b12
000828162 7001_ $$0P:(DE-Juel1)136801$$aZhao, Defeng$$b13
000828162 7001_ $$0P:(DE-Juel1)4528$$aKiendler-Scharr, Astrid$$b14
000828162 7001_ $$0P:(DE-Juel1)16346$$aMentel, Thomas F.$$b15
000828162 7001_ $$0P:(DE-HGF)0$$aRudich, Yinon$$b16
000828162 7001_ $$0P:(DE-HGF)0$$aHallquist, Mattias$$b17
000828162 7001_ $$0P:(DE-HGF)0$$aDoussin, Jean-Francois$$b18
000828162 7001_ $$0P:(DE-HGF)0$$aMaenhaut, Willy$$b19
000828162 7001_ $$0P:(DE-HGF)0$$aBäck, Jaana$$b20
000828162 7001_ $$0P:(DE-HGF)0$$aPetäjä, Tuukka$$b21
000828162 7001_ $$0P:(DE-HGF)0$$aWenger, John$$b22
000828162 7001_ $$0P:(DE-HGF)0$$aKulmala, Markku$$b23
000828162 7001_ $$0P:(DE-HGF)0$$aKalberer, Markus$$b24$$eCorresponding author
000828162 773__ $$0PERI:(DE-600)2615211-3$$a10.1038/srep35038$$gVol. 6, no. 1, p. 35038$$n1$$p35038$$tScientific reports$$v6$$x2045-2322$$y2016
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