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005     20230426083143.0
024 7 _ |2 doi
|a 10.1103/PhysRevB.95.094409
024 7 _ |2 ISSN
|a 0163-1829
024 7 _ |2 ISSN
|a 0556-2805
024 7 _ |2 ISSN
|a 1094-1622
024 7 _ |2 ISSN
|a 1095-3795
024 7 _ |2 ISSN
|a 1098-0121
024 7 _ |2 ISSN
|a 1550-235X
024 7 _ |2 ISSN
|a 2469-9950
024 7 _ |2 ISSN
|a 2469-9969
024 7 _ |2 Handle
|a 2128/13942
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037 _ _ |a FZJ-2017-02199
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100 1 _ |0 P:(DE-Juel1)156533
|a Esat, Taner
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245 _ _ |a Quantum interference effects in molecular spin hybrids
260 _ _ |a Woodbury, NY
|b Inst.
|c 2017
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520 _ _ |a We have studied by means of low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS) single molecular spin hybrids formed upon chemisorbing a polycyclic aromatic, threefold symmetric hydrocarbon molecule on Co(111) nanoislands. The spin-dependent hybridization between the Co d states and the π orbitals of the molecule leads to a spin-imbalanced electronic structure of the chemisorbed organic molecule. Spin-sensitive measurements reveal that the spin polarization shows intramolecular variations among the different aromatic rings in spite of the highly symmetric adsorption geometry promoted by symmetry matching of the threefold symmetric molecule and the sixfold symmetric Co(111) lattice. Hence the varying degree of spin polarization on the organic molecule does not stem from a different hybridization of the aromatic rings with the Co atoms, but is proposed to be a consequence of the superposition of the spin polarization of the molecule and the spatially modulated spin polarization of the spin-dependent quantum interference pattern of the Co(111) surface state.
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542 _ _ |i 2017-03-09
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542 _ _ |i 2018-03-09
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700 1 _ |0 P:(DE-Juel1)130948
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773 _ _ |a 10.1103/PhysRevB.95.094409
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