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| Hauptseite > Publikationsdatenbank > Repulsive Interactions Induced by Specific Adsorption: Anomalous Step Diffusivity and Inadequacy of Nearest-Neighbor Ising Model (Part II Theory) > print |
| Hauptseite > Publikationsdatenbank > Repulsive Interactions Induced by Specific Adsorption: Anomalous Step Diffusivity and Inadequacy of Nearest-Neighbor Ising Model (Part II Theory) > print |
| 001 | 828441 | ||
| 005 | 20210129230108.0 | ||
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| 245 | _ | _ | |a Repulsive Interactions Induced by Specific Adsorption: Anomalous Step Diffusivity and Inadequacy of Nearest-Neighbor Ising Model (Part II Theory) |
| 260 | _ | _ | |a Amsterdam |c 2017 |b Elsevier |
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| 520 | _ | _ | |a This is Part II of two closely related papers, where we show that the strong repulsive interaction caused by specifically adsorbed anions leads to a failure of the nearest-neighbor Ising model to describe structures on electrode surfaces. In this part, an analytical form of the step diffusivity is derived in terms of nearest and next-nearest neighbor interactions for steps with a mean direction along 〈110〉〈110〉 (the close-packed direction). With the help of a further analytical expression for the diffusivity of steps with 〈100〉〈100〉 mean orientation a simple scheme is developed whereby the nearest and next-nearest interaction energies can be extracted from the experimental values for the diffusivity along the 〈110〉〈110〉- and 〈100〉〈100〉-directions. The method is applicable to repulsive and attractive next-nearest neighbor interactions, both for surfaces in vacuum and in contact with an electrolyte. An example is presented in Part I, where we apply our approach to Au(100) in Br--, Cl-- and SO42—containing electrolytes. |
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| 700 | 1 | _ | |a Giesen, Margret |0 P:(DE-Juel1)4744 |b 1 |e Corresponding author |
| 700 | 1 | _ | |a Al-Shakran, Mohammad |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Kibler, Ludwig A. |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Jacob, Timo |0 P:(DE-HGF)0 |b 4 |
| 773 | _ | _ | |a 10.1016/j.susc.2016.03.022 |g Vol. 659, p. 52 - 57 |0 PERI:(DE-600)1479030-0 |p 52 - 57 |t Surface science |v 659 |y 2017 |x 0039-6028 |
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