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@ARTICLE{Henneke:828750,
      author       = {Henneke, Caroline and Felter, Janina and Schwarz, Daniel
                      and Tautz, F. S. and Kumpf, Christian},
      title        = {{C}ontrolling the growth of multiple ordered
                      heteromolecular phases by utilizing intermolecular
                      repulsion},
      journal      = {Nature materials},
      volume       = {16},
      issn         = {1476-4660},
      address      = {Basingstoke},
      publisher    = {Nature Publishing Group},
      reportid     = {FZJ-2017-02616},
      pages        = {628–633},
      year         = {2017},
      abstract     = {Metal/organic interfaces and their structural, electronic,
                      spintronic and thermodynamic properties have been
                      investigated intensively, aiming to improve and develop
                      future electronic devices. In this context, heteromolecular
                      phases add new design opportunities simply by combining
                      different molecules. However, controlling the desired phases
                      in such complex systems is a challenging task. Here, we
                      report an effective way of steering the growth of a
                      bimolecular system composed of adsorbate species with
                      opposite intermolecular interactions—repulsive and
                      attractive, respectively. The repulsive species forms a
                      two-dimensional lattice gas, the density of which controls
                      which crystalline phases are stable. Critical gas phase
                      densities determine the constant-area phase diagram that
                      describes our experimental observations, including eutectic
                      regions with three coexisting phases. We anticipate the
                      general validity of this type of phase diagram for binary
                      systems containing two-dimensional gas phases, and also show
                      that the density of the gas phase allows engineering of the
                      interface structure.},
      cin          = {PGI-3 / JARA-FIT},
      ddc          = {610},
      cid          = {I:(DE-Juel1)PGI-3-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
      pid          = {G:(DE-HGF)POF3-143},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000402017000010},
      pubmed       = {pmid:28272503},
      doi          = {10.1038/nmat4858},
      url          = {https://juser.fz-juelich.de/record/828750},
}