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000828969 1001_ $$0P:(DE-HGF)0$$aWagner, Ralf$$b0$$eCorresponding author
000828969 245__ $$aMagnesium-based additives for the cathode slurry to enable high voltage application of lithium-ion batteries
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000828969 520__ $$aThe kinetic stabilization of the cathode/electrolyte interface is essential to enhance cycle life and safety of lithium-ion batteries at high voltage application. The addition of only 2 wt.% Mg powder to the cathode slurry were found to significantly increase the cycle life of LiNi1/3Co1/3Mn1/3O2/Li half cells upon cycling to 4.6 V vs. Li/Li+, in terms of higher capacity retention, less parasitic reactions and less self-discharge. The presence of dissolved Mg2+ cations in the electrolyte during formation of the cell lead to an increased hydrolysis of the conducting salt LiPF6 and the formation of stable and effective LiPFxOy/Mg(PFxOy)2 species on the charged cathode surface.
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000828969 7001_ $$0P:(DE-HGF)0$$aGallus, Dennis R.$$b4
000828969 7001_ $$0P:(DE-HGF)0$$aAmereller, Marius$$b5
000828969 7001_ $$0P:(DE-HGF)0$$aKorth, Martin$$b6
000828969 7001_ $$0P:(DE-Juel1)171204$$aCekic-Laskovic, Isidora$$b7$$ufzj
000828969 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b8$$eCorresponding author$$ufzj
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