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@ARTICLE{Wagner:828969,
      author       = {Wagner, Ralf and Kraft, Vadim and Streipert, Benjamin and
                      Kasnatscheew, Johannes and Gallus, Dennis R. and Amereller,
                      Marius and Korth, Martin and Cekic-Laskovic, Isidora and
                      Winter, Martin},
      title        = {{M}agnesium-based additives for the cathode slurry to
                      enable high voltage application of lithium-ion batteries},
      journal      = {Electrochimica acta},
      volume       = {228},
      issn         = {0013-4686},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2017-02789},
      pages        = {9 - 17},
      year         = {2017},
      abstract     = {The kinetic stabilization of the cathode/electrolyte
                      interface is essential to enhance cycle life and safety of
                      lithium-ion batteries at high voltage application. The
                      addition of only 2 $wt.\%$ Mg powder to the cathode slurry
                      were found to significantly increase the cycle life of
                      LiNi1/3Co1/3Mn1/3O2/Li half cells upon cycling to 4.6 V vs.
                      Li/Li+, in terms of higher capacity retention, less
                      parasitic reactions and less self-discharge. The presence of
                      dissolved Mg2+ cations in the electrolyte during formation
                      of the cell lead to an increased hydrolysis of the
                      conducting salt LiPF6 and the formation of stable and
                      effective LiPFxOy/Mg(PFxOy)2 species on the charged cathode
                      surface.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000395211600002},
      doi          = {10.1016/j.electacta.2017.01.029},
      url          = {https://juser.fz-juelich.de/record/828969},
}