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@ARTICLE{Meister:828973,
author = {Meister, Paul and Fromm, Olga and Rothermel, Sergej and
Kasnatscheew, Johannes and Winter, Martin and Placke,
Tobias},
title = {{S}odium-{B}ased vs. {L}ithium-{B}ased {D}ual-{I}on
{C}ells: {E}lectrochemical {S}tudy of {A}nion
{I}ntercalation/{D}e-{I}ntercalation into/from {G}raphite
and {M}etal {P}lating/{D}issolution {B}ehavior},
journal = {Electrochimica acta},
volume = {228},
issn = {0013-4686},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2017-02790},
pages = {18 - 27},
year = {2017},
abstract = {Energy storage systems utilizing a simultaneous
intercalation of anions into a graphite host structure at
the positive electrode and intercalation/insertion/reduction
or deposition of cations at the negative electrode during
charge, were introduced under the term dual-ion cells,
recently. In this work, the electrochemical intercalation of
TFSI− anions into graphite has been studied in
sodium‐based dual‐ion cells (SDICs) at different upper
cut‐off potentials varying between 4.5 V and 4.7 V vs.
Na/Na+. Electrochemical characteristics of SDICs, including
the reversible capacity, Coulombic efficiency, energy
efficiency and onset potentials for anion intercalation,
were evaluated in comparison to the lithium-based dual-ions
cells (LDICs). A stable charge/discharge cycling performance
over 500 cycles has been found for SDICs providing a
specific capacity of ≈ 32 mAh g‐1 and a Coulombic
efficiency exceeding $99\%$ at an upper cut‐off potential
of 4.7 V vs. Na/Na+ at the graphite cathode. By the addition
of the electrolyte additive ethylene sulfite (ES), an
increase of the reversible capacity to ≈ 46 mAh g‐1 was
achieved. Furthermore, possible reasons for the overall
inferior cycling performance in terms of capacity for SDICs
as compared to LDICs such as an increased overpotential for
plating/stripping of Na+ ions as compared to Li+ ions are
discussed. In this respect, we also found that the addition
of ethylene sulfite particularly decreases the
overpotentials for the metal plating process, which at least
partially explains the enhanced reversible capacity in LDICs
and SDICs by using ES as electrolyte additive.},
cin = {IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000395211600003},
doi = {10.1016/j.electacta.2017.01.034},
url = {https://juser.fz-juelich.de/record/828973},
}