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| 024 | 7 | _ | |a 10.1016/j.elecom.2016.08.003 |2 doi |
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| 100 | 1 | _ | |a Meister, Paul |0 P:(DE-Juel1)172048 |b 0 |u fzj |
| 245 | _ | _ | |a New insights into the uptake/release of FTFSI − anions into graphite by means of in situ powder X-ray diffraction |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2016 |b Elsevier Science |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a The redox-amphoteric character of graphite enables its utilization as intercalation host for various types of cations and anions to form either donor-type or acceptor-type graphite intercalation compounds (GICs), respectively. While the donor-type GIC LiC6 is commonly used in the field of lithium ion batteries, acceptor-type GICs were suggested for application in dual-ion cells. In this contribution, the electrochemical intercalation/de-intercalation of fluorosulfonyl-(trifluoromethanesulfonyl) imide (FTFSI−) anions into graphite was studied for dual-ion cells during a cyclic voltammetry experiment using in situ powder X-ray diffraction. For the GICs, a series of most dominant stages could be assigned and the periodic repeat distance as well as the FTFSI− gallery height/gallery expansion were determined. The obtained dominant stage numbers of the formed GICs were correlated to cell voltage ranges. Upon charge, a transition of the different stages was observed, while upon discharge stage 1 was still preserved for a broad voltage range. These novel findings indicate different mechanisms for the uptake and release of the anions. |
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| 700 | 1 | _ | |a Schmuelling, Guido |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Winter, Martin |0 P:(DE-Juel1)166130 |b 2 |e Corresponding author |u fzj |
| 700 | 1 | _ | |a Placke, Tobias |0 P:(DE-HGF)0 |b 3 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.elecom.2016.08.003 |g Vol. 71, p. 52 - 55 |0 PERI:(DE-600)2027290-X |p 52 - 55 |t Electrochemistry communications |v 71 |y 2016 |x 1388-2481 |
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