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@ARTICLE{Sun:829533,
author = {Sun, X. and Klapper, A. and Su, Y. and Nemkovski, K. and
Wildes, A. and Bauer, H. and Köhler, O. and Schilmann, A.
and Tremel, W. and Petracic, O. and Brückel, Th.},
title = {{M}agnetism of monomer {M}n{O} and heterodimer
{F}e{P}t@{M}n{O} nanoparticles},
journal = {Physical review / B},
volume = {95},
number = {13},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2017-03218},
pages = {134427},
year = {2017},
abstract = {We report about the magnetic properties of
antiferromagnetic (AF) MnO nanoparticles (NPs) with
different sizes (6–19 nm). Using a combination of
polarized neutron scattering and magnetometry, we were able
to resolve previously observed peculiarities. Magnetometry,
on the one hand, reveals a peak in the zero-field-cooled
(ZFC) magnetization curves at low temperatures (∼25 K) but
no feature around the Néel temperature at 118 K. On the
other hand, polarized neutron scattering shows the expected
behavior of the AF order parameter vanishing around 118 K.
Moreover, hysteresis curves measured at various temperatures
reveal an exchange-bias effect, indicating a coupling of an
AF core to a ferromagnetic (FM)-like shell. ZFC data
measured at various fields exclude a purely
superparamagnetic (SPM) scenario. We conclude that the
magnetic behavior of MnO particles can be explained by a
superposition of SPM-like thermal fluctuations of the
AF-Néel vector inside the AF core and a magnetic coupling
to a ferrimagnetic Mn2O3 or Mn3O4 shell. In addition, we
have studied heterodimer (“Janus”) particles, where a FM
FePt particle is attached to the AF MnO particle. Via the
exchange-bias effect, the magnetic moment of the FePt
subunit is stabilized by the MnO.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS (München) ; Jülich
Centre for Neutron Science JCNS (München) ; JCNS-FRM-II},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)DNS-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000399789000004},
doi = {10.1103/PhysRevB.95.134427},
url = {https://juser.fz-juelich.de/record/829533},
}