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@ARTICLE{He:830153,
      author       = {Heß, Volkmar and Friedrich, Rico and Matthes, Frank and
                      Caciuc, Vasile and Atodiresei, Nicolae and Bürgler, Daniel
                      E and Blügel, Stefan and Schneider, Claus Michael},
      title        = {{M}agnetic subunits within a single molecule–surface
                      hybrid},
      journal      = {New journal of physics},
      volume       = {19},
      number       = {5},
      issn         = {1367-2630},
      address      = {[Bad Honnef]},
      publisher    = {Dt. Physikalische Ges.},
      reportid     = {FZJ-2017-03730},
      pages        = {053016 -},
      year         = {2017},
      abstract     = {Magnetic molecule–surface hybrids are ideal building
                      blocks for molecular spintronic devices due to their
                      appealing tailorable magnetic properties and nanoscale size.
                      So far, assemblies of interacting molecular-surface hybrids
                      needed for spintronic functionality were generated by
                      depositing aromatic molecules onto transition-metal
                      surfaces, resulting in a random arrangement of hybrid
                      magnets due to the inherent and strong hybridization. Here,
                      we demonstrate the formation of multiple intramolecular
                      subunits within a single molecule–surface hybrid by means
                      of spin-polarized scanning tunneling microscopy experiments
                      and ab initio density functional theory calculations. This
                      novel effect is realized by depositing a polycyclic aromatic
                      molecule on a magnetic surface. A highly asymmetric chiral
                      adsorption position induces different structural,
                      electronic, and magnetic properties in each aromatic ring of
                      the molecule. In particular, the induced molecular spin
                      polarization near the Fermi energy varies among the rings
                      due to site- and spin-dependent molecule–surface
                      hybridization. Our results showcase a possible organic
                      chemistry route of tailoring geometrically well-defined
                      assemblies of magnetically distinguishable subunits in
                      molecule–surface hybrids.},
      cin          = {PGI-6 / IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
      ddc          = {530},
      cid          = {I:(DE-Juel1)PGI-6-20110106 / I:(DE-Juel1)IAS-1-20090406 /
                      I:(DE-Juel1)PGI-1-20110106 / $I:(DE-82)080009_20140620$ /
                      $I:(DE-82)080012_20140620$},
      pnm          = {522 - Controlling Spin-Based Phenomena (POF3-522)},
      pid          = {G:(DE-HGF)POF3-522},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000402532100002},
      doi          = {10.1088/1367-2630/aa6ece},
      url          = {https://juser.fz-juelich.de/record/830153},
}