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@PHDTHESIS{Mller:830200,
author = {Müller, Mathias Christian Thomas David},
title = {{S}pin-wave excitations and electron-magnonscattering in
elementary ferromagnets from $\textit{ab initio}4 many-body
perturbation theory},
volume = {146},
school = {RWTH Aachen},
type = {Dr.},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek Verlag},
reportid = {FZJ-2017-03774},
isbn = {978-3-95806-242-9},
series = {Schriften des Forschungszentrums Jülich. Reihe
Schlüsseltechnologien / Key Technologies},
pages = {VI, 174 S.},
year = {2017},
note = {RWTH Aachen, Diss., 2017},
abstract = {In this thesis, an $\textit{ab initio}$ theoretical
framework for the investigation of spin excitations and the
electron-magnon scattering is developed within many-body
perturbation theory and implemented in the full-potential
linearized augmented-plane-wave method. The spin
excitations, including single-particle Stoner excitations
and collective spin waves, are accessible through the
magnetic response function, which is obtained by the
solution of a Bethe-Salpeter equation employing four-point
functions. These four-point functions are represented in a
Wannier-function basis, which allows to exploit the
short-range behavior of the screened interaction in metallic
systems by truncating the matrices in real space. The spin
excitation spectrum of ferromagnetic materials contains an
acoustic magnon mode whose energy, in the absence of
spin-orbit coupling, vanishes in the long-wavelength limit
as a consequence of the spontaneously broken spin-rotation
symmetry in these materials according to the Goldstone
theorem. However, in numerical realizations of the magnetic
response function the acoustic magnon mode exhibits a small
but finite gap in the Goldstone-mode limit. We investigate
this violation of the Goldstone theorem and present
anapproach that implements the magnetic response function
employing the properly renormalized Green function instead
of the Kohn-Sham one. This much more expensive approach
shows a substantial reduction of the gap error. In addition,
we discuss a correction scheme motivated by the one-band
Hubbard model that cures the fundamental inconsistency of
using the Kohn-Sham Green function by adjusting the exchange
splitting. We present corrected magnon spectra for the
elementary ferromagnets iron, cobalt, and nickel. We then
employ the T-matrix approach for the description of the
electron-magnon interaction within the GT approximation,
which can be combined with the GW approximation without the
need of double-counting corrections. The multiple-scattering
T matrix is part of the four-point magnetic response
function and describes the correlated propagation of
electron-hole pairs with opposite spins from which the
collective spin excitations arise. We apply the GT
approximation to Fe, Co, and Ni and present renormalized
spectral functions. The GT approximation leads to a
pronounced spin-dependent lifetime broadening of the
quasiparticle states to the extent that the quasiparticle
character is virtually lost in certain energy regions. In
iron, the spectral functions exhibit an additional
quasiparticle peak indicating the emergence of a new
quasiparticle. We discuss the features of this quasiparticle
state that forms out of a superposition of single-particle
and magnon excitations. In addition, we find kink structures
in the quasiparticle dispersion of free-electron-like bands
of cobalt and nickel.},
cin = {PGI-1 / IAS-1 / JARA-FIT / JARA-HPC},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)3 / PUB:(DE-HGF)11},
url = {https://juser.fz-juelich.de/record/830200},
}