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@ARTICLE{Passens:830424,
author = {Passens, Michael and Caciuc, V. and Atodiresei, N. and
Feuerbacher, Michael and Moors, M. and Dunin-Borkowski,
Rafal and Blügel, S. and Waser, R. and Karthäuser, S.},
title = {{I}nterface-driven formation of a two-dimensional
dodecagonal fullerene quasicrystal},
journal = {Nature Communications},
volume = {8},
issn = {2041-1723},
address = {London},
publisher = {Nature Publishing Group},
reportid = {FZJ-2017-03973},
pages = {15367},
year = {2017},
abstract = {Since their discovery, quasicrystals have attracted
continuous research interest due to their unique structural
and physical properties. Recently, it was demonstrated that
dodecagonal quasicrystals could be used as bandgap materials
in next-generation photonic devices. However, a full
understanding of the formation mechanism of quasicrystals is
necessary to control their physical properties. Here we
report the formation of a two-dimensional dodecagonal
fullerene quasicrystal on a Pt3Ti(111) surface, which can be
described in terms of a square–triangle tiling. Employing
density functional theory calculations, we identify the
complex adsorption energy landscape of the Pt-terminated
Pt3Ti surface that is responsible for the quasicrystal
formation. We demonstrate the presence of
quasicrystal-specific phason strain, which provides the
degree of freedom required to accommodate the
quasicrystalline structure on the periodic substrate. Our
results reveal detailed insight into an interface-driven
formation mechanism and open the way to the creation of
tailored fullerene quasicrystals with specific physical
properties.},
cin = {IAS-1 / PGI-1 / PGI-7 / JARA-FIT / JARA-HPC / PGI-5 /
ER-C-1},
ddc = {500},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$ /
$I:(DE-82)080012_20140620$ / I:(DE-Juel1)PGI-5-20110106 /
I:(DE-Juel1)ER-C-1-20170209},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142) / 143 -
Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-142 / G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000401907600001},
pubmed = {pmid:28530242},
doi = {10.1038/ncomms15367},
url = {https://juser.fz-juelich.de/record/830424},
}