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@ARTICLE{Kaus:834095,
author = {Kaus, Maximilian and Guin, Marie and Yavuz, Murat and
Knapp, Michael and Tietz, Frank and Guillon, Olivier and
Ehrenberg, Helmut and Indris, Sylvio},
title = {{F}ast {N}a+ {I}on {C}onduction in {NASICON}-{T}ype
{N}a3.4{S}c2({S}i{O}4)0.4({PO}4 )2.6 {O}bserved by 23{N}a
{NMR} {R}elaxometry},
journal = {The journal of physical chemistry / C},
volume = {121},
number = {3},
issn = {1932-7447},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2017-04096},
pages = {1449 - 1454},
year = {2017},
abstract = {The bulk diffusion of Na in Na3.4Sc2(SiO4)0.4(PO4)2.6 was
investigated by 23Na NMR relaxometry in the temperature
range from 250 to 670 K. These measurements reveal fast Na
diffusion with hopping rates of 3 × 108 s–1 for the Na+
ions at 350 K and activation barriers for single Na+ ion
jumps of (0.20 ± 0.01) eV. From these values a diffusion
coefficient of D = 6.4 × 10–12 m2/s and a Na ion
conductivity of σNa = 4 mS/cm (both at 350 K) can be
estimated. Measurements on two samples, one stored in air
and one stored in Ar, do not show significant differences,
which reveals that these NMR measurements are probing the
bulk diffusion while conductivity measurements usually are
also influenced by grain boundaries that can be affected by
the moisture level during storage.},
cin = {IEK-12 / IEK-1 / JARA-ENERGY},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217 / I:(DE-Juel1)IEK-1-20101013 /
$I:(DE-82)080011_20140620$},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000393008900009},
doi = {10.1021/acs.jpcc.6b10523},
url = {https://juser.fz-juelich.de/record/834095},
}