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@ARTICLE{Guin:834097,
author = {Guin, Marie and Indris, S. and Kaus, M. and Ehrenberg, H.
and Tietz, F. and Guillon, O.},
title = {{S}tability of {NASICON} materials against water and {CO} 2
uptake},
journal = {Solid state ionics},
volume = {302},
issn = {0167-2738},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2017-04098},
pages = {102 - 106},
year = {2017},
abstract = {The stability in ambient conditions of a scandium-based
NASICON material, Na3.4Sc2Si0.4P2.6O12, was investigated
using impedance spectroscopy, thermogravimetry/differential
scanning calorimetry (TG/DSC) and multinuclear magic angle
spinning nuclear magnetic resonance spectroscopy (MAS NMR).
The presence of H2O and CO2 in samples stored in ambient air
could be evidenced as well as its impact on the ionic
conductivity of the samples.The detected amounts of water
and CO2 in the samples had no influence on the measured
conductivities at room temperature, which confirmed the
absence of protonic conduction in hydrated samples. A loss
of conductivity during heating of hydrated samples was due
to a loss of contact between the ceramic and the electrode
used for the conductivity measurement.The recommendation for
handling of NASICON-type materials is therefore: samples
require storage in an Ar-filled glove box or in a dry
environment to avoid artefacts during high temperature
measurements. Nevertheless, the stability of the
NASICON-type materials is confirmed since their conductivity
is not affected by the moisture.},
cin = {IEK-1 / IEK-12 / JARA-ENERGY},
ddc = {530},
cid = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-12-20141217 /
$I:(DE-82)080011_20140620$},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000397688300020},
doi = {10.1016/j.ssi.2016.11.006},
url = {https://juser.fz-juelich.de/record/834097},
}