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@ARTICLE{Wang:834126,
author = {Wang, Rui and Di, Zhen-Yu and M?ller-Buschbaum, Peter and
Frielinghaus, Henrich},
title = {{E}ffect of {PCBM} additive on morphology and
optoelectronic properties of {P}3{HT}- b -{PS} films},
journal = {Polymer},
volume = {121},
issn = {0032-3861},
address = {Oxford},
publisher = {Elsevier Science},
reportid = {FZJ-2017-04125},
pages = {173–182},
year = {2017},
abstract = {Thin blend films of the diblock copolymer
poly(3-hexylthiophene-2,5-diyl)-block-polystyrene
(P3HT-b-PS) and phenyl-C61-butyric acid methyl ester (PCBM)
are prepared and investigated. The morphology of films with
9, 25, 33, 50, 58 and $67\%$ PCBM weight fraction is
determined. The surface topography is probed with optical
microscopy and atomic force microscopy whereas the lateral
inner structures are determined using grazing incidence
small angle neutron scattering (GISANS). Grazing incidence
X-ray diffraction (GI-XRD) shows a blend ratio dependence of
the P3HT crystallites orientation within the block copolymer
films. The thermodynamically favoured P3HT edge-on
orientation is suppressed upon increasing the PCBM content
from $9\%$ till $33\%$ while it recovers in samples with a
PCBM weight fraction above $50\%.$ PCBM tends to interact
with the PS block at low PCBM fractions and forms segregated
domains at a PCBM weight fraction higher than $50\%.$ The
addition of PCBM decreases the degree of lamellar structure
order and well-ordered hexagonal packed cylindrical
structures emerge in at a PCBM weight fraction of $67\%.$
Absorbance and photoluminescence measurements show the
relationship between morphology transformation and
optoelectronic properties. The phenomena reported here could
provide an alternative view for potential nanotechnology
applications.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6215 - Soft Matter, Health and Life Sciences (POF3-621) /
6G15 - FRM II / MLZ (POF3-6G15)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6215 /
G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)KWS1-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000405747100019},
doi = {10.1016/j.polymer.2017.06.016},
url = {https://juser.fz-juelich.de/record/834126},
}