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@ARTICLE{Kunkemller:834219,
author = {Kunkemöller, S. and Komleva, E. and Streltsov, S. V. and
Hoffmann, S. and Khomskii, D. I. and Steffens, P. and Sidis,
Y. and Schmalzl, K. and Braden, M.},
title = {{M}agnon dispersion in {C}a2{R}u1−x{T}ix{O}4: {I}mpact of
spin-orbit coupling and oxygen moments},
journal = {Physical review / B},
volume = {95},
number = {21},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2017-04201},
pages = {214408},
year = {2017},
abstract = {The magnon dispersion of Ca2RuO4 has been studied by
polarized and unpolarized neutron scattering experiments on
crystals containing 0, 1, and $10\%$ of Ti. Ti is inserted
in order to enable the growth of large, partially detwinned
crystals. One percent of Ti has a negligible impact on
structural and magnetic properties. Also for $10\%$ Ti
content magnetic properties still change very little, but
the insulating phase is stabilized up to at least 700 K and
structural distortions are reduced. The full dispersion of
transverse magnons studied for $1\%$ Ti substitution can be
well described by a conventional spin-wave model with
interaction and anisotropy parameters that agree with
density functional theory calculations. Spin-orbit coupling
strongly influences the magnetic excitations, as it is most
visible in large energies of the magnetic zone-center modes
arising from magnetic anisotropy. Additional modes appear at
low energy near the antiferromagnetic zone center and can be
explained by a sizable magnetic moment of 0.11 Bohr
magnetons, which the density functional theory calculations
find located on the apical oxygens. The energy and the
signal strength of the additional branch are well described
by taking into account this oxygen moment with weak
ferromagnetic coupling to the Ru moments.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS-ILL},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)JCNS-ILL-20110128},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-Juel1)ILL-IN12-20150421},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000403069600006},
doi = {10.1103/PhysRevB.95.214408},
url = {https://juser.fz-juelich.de/record/834219},
}