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@ARTICLE{Ghavami:834261,
      author       = {Ghavami, Ali and Winkler, Roland G.},
      title        = {{S}olvent {I}nduced {I}nversion of {C}ore-{S}hell
                      {M}icrogels},
      journal      = {ACS Macro Letters},
      volume       = {6},
      issn         = {2161-1653},
      address      = {Washington, DC},
      publisher    = {ACS},
      reportid     = {FZJ-2017-04243},
      pages        = {721 - 725},
      year         = {2017},
      abstract     = {The morphology of core–shell microgels under different
                      swelling conditions and as a function of the core–shell
                      thickness ratio is systematically characterized by mesoscale
                      hydrodynamic simulations. With increasing hydrophobic
                      interaction of the shell polymers, we observe drastic
                      morphological changes from a core–shell structure to an
                      inverted microgel, where the core is turned to the outside,
                      or a microgel with a patchy surface of core polymers
                      directly exposed to the environment. We establish a phase
                      diagram of the various morphologies. Moreover, we
                      characterize the polymer and microgel conformations. For
                      sufficiently thick shells, the changes of the shell size
                      upon increasing hydrophobic interactions are well described
                      by the Flory–Rehner theory. Additionally, this theory
                      provides a critical line in the phase diagram separating
                      core–shell structures from the distinct two other phases.
                      The appearing new phases provide a novel route to nano- and
                      microscale functionalized materials.},
      cin          = {IAS-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IAS-2-20090406},
      pnm          = {551 - Functional Macromolecules and Complexes (POF3-551)},
      pid          = {G:(DE-HGF)POF3-551},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000406087600016},
      doi          = {10.1021/acsmacrolett.7b00318},
      url          = {https://juser.fz-juelich.de/record/834261},
}