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@ARTICLE{Rupprecht:835978,
author = {Rupprecht, Christian and Wingen, Marcus and Potzkei, Janko
and Gensch, Thomas and Jaeger, Karl-Erich and Drepper,
Thomas},
title = {{A} novel {F}b{FP}-based biosensor toolbox for sensitive in
vivo determination of intracellular p{H}},
journal = {Journal of biotechnology},
volume = {258},
issn = {0168-1656},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2017-05103},
pages = {25-32},
year = {2017},
abstract = {The intracellular pH is an important modulator of various
bio(techno)logical processes such as enzymatic conversion of
metabolites or transport across the cell membrane. Changes
of intracellular pH due to altered proton distribution can
thus cause dysfunction of cellular processes. Consequently,
accurate monitoring of intracellular pH allows elucidating
the pH-dependency of (patho)physiological and
biotechnological processes. In this context, genetically
encoded biosensors represent a powerful tool to determine
intracellular pH values non-invasively and with high
spatiotemporal resolution.We have constructed a toolbox of
novel genetically encoded FRET-based pH biosensors (named
Fluorescence Biosensors for pH or FluBpH) that utilizes the
FMN-binding fluorescent protein EcFbFP as donor domain. In
contrast to many fluorescent proteins of the GFP family,
EcFbFP exhibits a remarkable tolerance towards acidic pH
(pKa ∼ 3.2). To cover the broad range of physiologically
relevant pH values, three EYFP variants exhibiting pKa
values of 5.7, 6.1 and 7.5 were used as pH-sensing FRET
acceptor domains. The resulting biosensors FluBpH 5.7,
FluBpH 6.1 and FluBpH 7.5 were calibrated in vitro and in
vivo to accurately evaluate their pH indicator properties.
To demonstrate the in vivo applicability of FluBpH, changes
of intracellular pH were ratiometrically measured in E. coli
cells during acid stress.},
cin = {ICS-4 / IMET},
ddc = {540},
cid = {I:(DE-Juel1)ICS-4-20110106 / I:(DE-Juel1)IMET-20090612},
pnm = {552 - Engineering Cell Function (POF3-552) / 581 -
Biotechnology (POF3-581)},
pid = {G:(DE-HGF)POF3-552 / G:(DE-HGF)POF3-581},
typ = {PUB:(DE-HGF)25},
pubmed = {pmid:28501596},
doi = {10.1016/j.jbiotec.2017.05.006},
url = {https://juser.fz-juelich.de/record/835978},
}