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@ARTICLE{Guo:836079,
author = {Guo, Fangwei and Wang, Guowei and Jiang, Zhiwei and Liu,
Yang and Zhao, Xiaofeng and Xiao, Ping},
title = {{G}rowth of carbon nanofibers/tubes by an in-situ
polymerization route without metal-catalyst},
journal = {Carbon},
volume = {100},
issn = {0008-6223},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2017-05203},
pages = {417 - 427},
year = {2016},
abstract = {An in-situ pyrolytic and polymerizable method was
investigated to grow carbon nano-fibers/tubes (CNF/CNT)
without metal-catalysts. The 3 mol $\%$ yttria-stabilized
zirconia hollow fiber membranes (3YSZ-HFM) were used as
supports for growing the CNF/CNT. The polyethersulfone (PES)
and polyvinylpyrrolidone (PVP) were used as polymer binders
and carbon sources. The as-grown CNF (formed at 1250 °C/4h)
had diameters of 50–100 nm and lengths of 1–50 μm, and
the length gradually decreased along radial direction of the
supports. The as-grown CNT (formed at 1450 °C/4h) were
shorter and larger in diameter. A novel solid-state
transformation mechanism was proposed, in which the carbon
black particles (CB) were the carbonized products of
PES/PVP, then the CB grew into the CNF/CNT. Thermal stresses
originated from sintering of CB itself and 3YSZ particles
were believed to be the driving forces that promoting the
CNT/CNF nucleation and growth. The thermal stresses of the
pure 3YSZ-HFM and 3YSZ/(CNF/CNT)-HFM were theoretically and
experimentally discussed base on linear elastic thoery and
Raman spectroscopy.},
cin = {IEK-1},
ddc = {540},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {113 - Methods and Concepts for Material Development
(POF3-113) / HITEC - Helmholtz Interdisciplinary Doctoral
Training in Energy and Climate Research (HITEC)
(HITEC-20170406)},
pid = {G:(DE-HGF)POF3-113 / G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000369961400048},
doi = {10.1016/j.carbon.2016.01.041},
url = {https://juser.fz-juelich.de/record/836079},
}