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@ARTICLE{Shams:836621,
author = {Shams, S. Fatemeh and Kashefi, Mehrdad and
Schmitz-Antoniak, Carolin},
title = {{S}tatistical approach of synthesize {C}o{F}e 2 {O} 4
nanoparticles to optimize their characteristics using
response surface methodology},
journal = {Journal of magnetism and magnetic materials},
volume = {432},
issn = {0304-8853},
address = {Amsterdam},
publisher = {North-Holland Publ. Co.},
reportid = {FZJ-2017-05694},
pages = {362 - 372},
year = {2017},
abstract = {The performance of magnetic nanoparticles in different
applications is severely depended on their size
characteristics, so the study of effective parameters on
these properties can play significant roles in
qualifications of nanoparticles. In present work, some
important factors on size features of CoFe2O4
superparamagnetic nanoparticles include the mixing order of
synthesis components, the utilized reduction agents,
stabilization process, and chelating mechanisms were
investigated. Moreover, in order to optimize several
influential factors such as the temperature, pH, and cation
ratio of reaction, the experimental design was done by using
central composite design method of response surface
methodology. The simultaneous effects on the particles size
and their size distribution were investigated by different
methods i.e. dynamic light scattering, X-ray diffraction,
Fourier transform inferred spectroscopy, vibration sample
magnetometer, and transmission electron microscopy. Results
demonstrated the mixing order of reduction agent to salt
solution and also the employing of NH4OH as a reduction
agent could cause to significant decreasing of particles
size and size distribution. Furthermore, the nitric acid
could stabilize and chelate nanoparticles more appropriate
than citric acid. Based on the optimization results, the
quadratic polynomial models were fitted on the responses
which could predict their amounts, while temperature, pH,
and their interactions had higher effectiveness. In
addition, the optimum amounts of particle size (14 nm) and
size distribution (4.61 nm) were achieved while temperature,
pH, and cation ratio amounts are equal to 89.82 °C, 11, and
0.52, respectively},
cin = {PGI-6},
ddc = {530},
cid = {I:(DE-Juel1)PGI-6-20110106},
pnm = {522 - Controlling Spin-Based Phenomena (POF3-522)},
pid = {G:(DE-HGF)POF3-522},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000399601600054},
doi = {10.1016/j.jmmm.2017.02.017},
url = {https://juser.fz-juelich.de/record/836621},
}