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000836763 0247_ $$2doi$$a10.1002/2016JD025767
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000836763 1001_ $$00000-0001-6205-9698$$aTzompa-Sosa, Z. A.$$b0$$eCorresponding author
000836763 245__ $$aRevisiting global fossil fuel and biofuel emissions of ethane
000836763 260__ $$aHoboken, NJ$$bWiley$$c2017
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000836763 520__ $$aRecent measurements over the Northern Hemisphere indicate that the long-term decline in the atmospheric burden of ethane (C2H6) has ended and the abundance increased dramatically between 2010 and 2014. The rise in C2H6 atmospheric abundances has been attributed to oil and natural gas extraction in North America. Existing global C2H6 emission inventories are based on outdated activity maps that do not account for current oil and natural gas exploitation regions. We present an updated global C2H6 emission inventory based on 2010 satellite-derived CH4 fluxes with adjusted C2H6 emissions over the U.S. from the National Emission Inventory (NEI 2011). We contrast our global 2010 C2H6 emission inventory with one developed for 2001. The C2H6 difference between global anthropogenic emissions is subtle (7.9 versus 7.2 Tg yr−1), but the spatial distribution of the emissions is distinct. In the 2010 C2H6 inventory, fossil fuel sources in the Northern Hemisphere represent half of global C2H6 emissions and 95% of global fossil fuel emissions. Over the U.S., unadjusted NEI 2011 C2H6 emissions produce mixing ratios that are 14–50% of those observed by aircraft observations (2008–2014). When the NEI 2011 C2H6 emission totals are scaled by a factor of 1.4, the Goddard Earth Observing System Chem model largely reproduces a regional suite of observations, with the exception of the central U.S., where it continues to underpredict observed mixing ratios in the lower troposphere. We estimate monthly mean contributions of fossil fuel C2H6 emissions to ozone and peroxyacetyl nitrate surface mixing ratios over North America of ~1% and ~8%, respectively.
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000836763 7001_ $$0P:(DE-HGF)0$$aMahieu, E.$$b1
000836763 7001_ $$0P:(DE-Juel1)168550$$aFranco, B.$$b2$$ufzj
000836763 7001_ $$0P:(DE-HGF)0$$aKeller, C. A.$$b3
000836763 7001_ $$0P:(DE-HGF)0$$aTurner, A. J.$$b4
000836763 7001_ $$0P:(DE-HGF)0$$aHelmig, D.$$b5
000836763 7001_ $$00000-0002-5230-3527$$aFried, A.$$b6
000836763 7001_ $$00000-0002-2156-031X$$aRichter, D.$$b7
000836763 7001_ $$0P:(DE-HGF)0$$aWeibring, P.$$b8
000836763 7001_ $$0P:(DE-HGF)0$$aWalega, J.$$b9
000836763 7001_ $$0P:(DE-HGF)0$$aYacovitch, T. I.$$b10
000836763 7001_ $$0P:(DE-HGF)0$$aHerndon, S. C.$$b11
000836763 7001_ $$0P:(DE-HGF)0$$aBlake, D. R.$$b12
000836763 7001_ $$0P:(DE-HGF)0$$aHase, F.$$b13
000836763 7001_ $$0P:(DE-HGF)0$$aHannigan, J. W.$$b14
000836763 7001_ $$0P:(DE-HGF)0$$aConway, S.$$b15
000836763 7001_ $$0P:(DE-HGF)0$$aStrong, K.$$b16
000836763 7001_ $$0P:(DE-HGF)0$$aSchneider, M.$$b17
000836763 7001_ $$0P:(DE-HGF)0$$aFischer, E. V.$$b18
000836763 773__ $$0PERI:(DE-600)2016800-7$$a10.1002/2016JD025767$$gVol. 122, no. 4, p. 2493 - 2512$$n4$$p2493 - 2512$$tJournal of geophysical research / Atmospheres$$v122$$x2169-897X$$y2017
000836763 8564_ $$uhttps://juser.fz-juelich.de/record/836763/files/Tzompa-Sosa_et_al-2017-Journal_of_Geophysical_Research__Atmospheres.pdf$$yPublished on 2017-02-28. Available in OpenAccess from 2017-08-28.
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