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@ARTICLE{Gaudenzi:836896,
      author       = {Gaudenzi, R. and Misiorny, M. and Burzurí, E. and
                      Wegewijs, M. R. and van der Zant, H. S. J.},
      title        = {{T}ransport mirages in single-molecule devices},
      journal      = {The journal of chemical physics},
      volume       = {146},
      number       = {9},
      issn         = {1089-7690},
      address      = {Melville, NY},
      publisher    = {American Institute of Physics},
      reportid     = {FZJ-2017-05928},
      pages        = {092330 -},
      year         = {2017},
      abstract     = {Molecular systems can exhibit a complex, chemically
                      tailorable inner structure which allows for targeting of
                      specific mechanical, electronic, and optical properties. At
                      the single-molecule level, two major complementary ways to
                      explore these properties are molecular quantum-dot
                      structures and scanning probes. This article outlines
                      comprehensive principles of electron-transport spectroscopy
                      relevant to both these approaches and presents a new,
                      high-resolution experiment on a high-spin single-molecule
                      junction exemplifying these principles. Such spectroscopy
                      plays a key role in further advancing our understanding of
                      molecular and atomic systems, in particular, the relaxation
                      of their spin. In this joint experimental and theoretical
                      analysis, particular focus is put on the crossover between
                      the resonant regime [single-electron tunneling] and the
                      off-resonant regime [inelastic electron (co)tunneling
                      spectroscopy (IETS)]. We show that the interplay of these
                      two processes leads to unexpected mirages of resonances not
                      captured by either of the two pictures alone. Although this
                      turns out to be important in a large fraction of the
                      possible regimes of level positions and bias voltages, it
                      has been given little attention in molecular transport
                      studies. Combined with nonequilibrium IETS—four-electron
                      pump-probe excitations—these mirages provide crucial
                      information on the relaxation of spin excitations. Our
                      encompassing physical picture is supported by a
                      master-equation approach that goes beyond weak coupling. The
                      present work encourages the development of a broader
                      connection between the fields of molecular quantum-dot and
                      scanning probe spectroscopy},
      cin          = {PGI-2 / JARA-FIT},
      ddc          = {540},
      cid          = {I:(DE-Juel1)PGI-2-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {141 - Controlling Electron Charge-Based Phenomena
                      (POF3-141)},
      pid          = {G:(DE-HGF)POF3-141},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000397312800032},
      doi          = {10.1063/1.4975767},
      url          = {https://juser.fz-juelich.de/record/836896},
}