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@ARTICLE{Zhang:837185,
      author       = {Zhang, Tong and de Meatza, Iratxe and Qi, Xin and Paillard,
                      Elie},
      title        = {{E}nabling steady graphite anode cycling with high voltage,
                      additive-free, sulfolane-based electrolyte: {R}ole of the
                      binder},
      journal      = {Journal of power sources},
      volume       = {356},
      issn         = {0378-7753},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2017-06164},
      pages        = {97 - 102},
      year         = {2017},
      abstract     = {We demonstrate here the possibility of operating both high
                      voltage spinel and high mass loading graphite electrodes in
                      a 1 M LiPF6 in SL/DMC (1/1, wt/wt) electrolyte without the
                      use of additive. A crucial point for practical graphite
                      electrode operation is the use of the cheaper and
                      environmentally friendly carboxymethyl cellulose
                      (CMC)/styrene-butadiene rubber (SBR) combination instead of
                      the PVDF-based electrodes used in most laboratory studies.
                      With this type of anode we also show the operation of a full
                      Li-ion cell operating at 4.5 V without any additive and show
                      that most of the Li+ transport limitation observed in
                      half-cells are in fact due to the Li metal counter
                      electrode. The anode binder influence is to be considered
                      for the development of high voltage electrolytes lacking
                      good intrinsic SEI building properties, as the anode binder
                      does not affect cathode performance, contrary to most
                      additives. It opens the route for further improvement by use
                      of SEI forming additives (molecular and salts), keeping in
                      mind the requirement for the cathode.},
      cin          = {IEK-12},
      ddc          = {620},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000402342700011},
      doi          = {10.1016/j.jpowsour.2017.04.073},
      url          = {https://juser.fz-juelich.de/record/837185},
}