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@ARTICLE{Adly:837530,
author = {Adly, Nouran and Feng, Lingyan and Krause, Kay and Mayer,
Dirk and Yakushenko, Alexey and Offenhäusser, Andreas and
Wolfrum, Bernhard},
title = {{F}lexible {M}icrogap {E}lectrodes by {D}irect {I}nkjet
{P}rinting for {B}iosensing {A}pplication},
journal = {Advanced biosystems},
volume = {1},
number = {3},
issn = {2366-7478},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2017-06418},
pages = {1600016 -},
year = {2017},
abstract = {A rapid fabrication method of microgap electrodes using
inkjet printing is described. In this approach, the lateral
spacing between two printed electrode lines is precisely
controlled down to 1 µm without any surface modification or
substrate patterning. The strong confinement, well below
typical resolution of inkjet printing, relies on complete
solvent evaporation between the printing of adjacent
electrode structures, which is achieved by controlling the
printing speed and temperature profiles. The feasibility of
this method is demonstrated by writing electrode structures
with two distinct inks, based on carbon and silver
nanoparticles, with comparable results. As an application
proof-of-principle, arrays of microgap electrodes are
fabricated using a carbon nanoparticle ink for
electrochemical detection based on redox-cycling, a
technique in which the sensitivity of the device depends on
the distance between the two electrodes. The redox-cycling
amplification of electrochemical signals is demonstrated and
it is shown that the printed microgap device can be used as
an electrochemical biosensor for the determination of human
immunodeficiency virus (HIV)-related single-stranded DNA.
This work presents a promising new approach for fabricating
low-cost and label-free redox-cycling biosensors using
all-inkjet-printed electrodes.},
cin = {ICS-8 / PGI-8},
ddc = {570},
cid = {I:(DE-Juel1)ICS-8-20110106 / I:(DE-Juel1)PGI-8-20110106},
pnm = {523 - Controlling Configuration-Based Phenomena (POF3-523)},
pid = {G:(DE-HGF)POF3-523},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000446956600003},
doi = {10.1002/adbi.201600016},
url = {https://juser.fz-juelich.de/record/837530},
}