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| Hauptseite > Publikationsdatenbank > The Effect of Surface Site Ensembles on the Activity and Selectivity of Ethanol Electrooxidation by Octahedral PtNiRh Nanoparticles > print |
| Hauptseite > Publikationsdatenbank > The Effect of Surface Site Ensembles on the Activity and Selectivity of Ethanol Electrooxidation by Octahedral PtNiRh Nanoparticles > print |
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| 024 | 7 | _ | |a 10.1002/ange.201702332 |2 doi |
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| 037 | _ | _ | |a FZJ-2017-06627 |
| 082 | _ | _ | |a 540 |
| 100 | 1 | _ | |a Erini, Nina |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a The Effect of Surface Site Ensembles on the Activity and Selectivity of Ethanol Electrooxidation by Octahedral PtNiRh Nanoparticles |
| 260 | _ | _ | |a Weinheim |c 2017 |b Wiley-VCH65543 |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Direct ethanol fuel cells are attractive power sources based on a biorenewable, high energy-density fuel. Their efficiency is limited by the lack of active anode materials which catalyze the breaking of the C−C bond coupled to the 12-electron oxidation to CO2. We report shape-controlled PtNiRh octahedral ethanol oxidation electrocatalysts with excellent activity and previously unachieved low onset potentials as low as 0.1 V vs. RHE, while being highly selective to complete oxidation to CO2. Our comprehensive characterization and in situ electrochemical ATR studies suggest that the formation of a ternary surface site ensemble around the octahedral Pt3Ni1Rhx nanoparticles plays a crucial mechanistic role for this behavior. |
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| 700 | 1 | _ | |a Beermann, Vera |0 P:(DE-HGF)0 |b 1 |
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| 700 | 1 | _ | |a Strasser, Peter |0 P:(DE-HGF)0 |b 6 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/ange.201702332 |g Vol. 129, no. 23, p. 6633 - 6638 |0 PERI:(DE-600)1479266-7 |n 23 |p 6633 - 6638 |t Angewandte Chemie |v 129 |y 2017 |x 0044-8249 |
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