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000837854 1001_ $$0P:(DE-HGF)0$$aReichel, Victoria$$b0
000837854 245__ $$aSingle crystalline superstructured stable single domain magnetite nanoparticles
000837854 260__ $$aLondon$$bNature Publishing Group$$c2017
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000837854 520__ $$aMagnetite nanoparticles exhibit magnetic properties that are size and organization dependent and, for applications that rely on their magnetic state, they usually have to be monodisperse. Forming such particles, however, has remained a challenge. Here, we synthesize 40 nm particles of magnetite in the presence of polyarginine and show that they are composed of 10 nm building blocks, yet diffract like single crystals. We use both bulk magnetic measurements and magnetic induction maps recorded from individual particles using off-axis electron holography to show that each 40 nm particle typically contains a single magnetic domain. The magnetic state is therefore determined primarily by the size of the superstructure and not by the sizes of the constituent sub-units. Our results fundamentally demonstrate the structure – property relationship in a magnetic mesoparticle.
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000837854 7001_ $$0P:(DE-Juel1)144926$$aKovács, András$$b1
000837854 7001_ $$0P:(DE-HGF)0$$aKumari, Monika$$b2
000837854 7001_ $$0P:(DE-HGF)0$$aBereczk-Tompa, Éva$$b3
000837854 7001_ $$0P:(DE-HGF)0$$aSchneck, Emanuel$$b4
000837854 7001_ $$0P:(DE-Juel1)162274$$aDiehle, Patrick$$b5
000837854 7001_ $$0P:(DE-HGF)0$$aPósfai, Mihály$$b6
000837854 7001_ $$0P:(DE-HGF)0$$aHirt, Ann M.$$b7
000837854 7001_ $$0P:(DE-Juel1)145413$$aDuchamp, Martial$$b8
000837854 7001_ $$0P:(DE-Juel1)144121$$aDunin-Borkowski, Rafal$$b9
000837854 7001_ $$0P:(DE-HGF)0$$aFaivre, Damien$$b10$$eCorresponding author
000837854 773__ $$0PERI:(DE-600)2615211-3$$a10.1038/srep45484$$gVol. 7, p. 45484 -$$p45484 -$$tScientific reports$$v7$$x2045-2322$$y2017
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